Journal Article PUBDB-2024-05578

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Out-of-equilibrium charge redistribution in a copper-oxide based superconductor by time-resolved X-ray photoelectron spectroscopy

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2024
Macmillan Publishers Limited, part of Springer Nature [London]

Scientific reports 14(1), 8775 () [10.1038/s41598-024-56440-4]
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Abstract: Charge-transfer excitations are of paramount importance for understanding the electronic structure of copper-oxide based high-temperature superconductors. In this study, we investigate the response of a $Bi_2Sr_2CaCu_2O_{8+\delta}$ crystal to the charge redistribution induced by an infrared ultrashort pulse. Element-selective time-resolved core-level photoelectron spectroscopy with a high energy resolution allows disentangling the dynamics of oxygen ions with different coordination and bonds thanks to their different chemical shifts. Our experiment shows that the O 1s component arising from the Cu–O planes is significantly perturbed by the infrared light pulse. Conversely, the apical oxygen, also coordinated with Sr ions in the Sr-O planes, remains unaffected. This result highlights the peculiar behavior of the electronic structure of the Cu–O planes. It also unlocks the way to study the out-of-equilibrium electronic structure of copper-oxide-based high-temperature superconductors by identifying the O 1s core-level emission originating from the oxygen ions in the Cu–O planes. This ability could be critical to gain information about the strongly-correlated electron ultrafast dynamical mechanisms in the Cu–O plane in the normal and superconducting phases.

Classification:

Contributing Institute(s):
  1. Laser Forschung und Entwicklung (FS-LA)
  2. DOOR-User (DOOR ; HAS-User)
  3. FLASH Wissenschaftlicher Nutzerbetrieb (FS-FLASH-O)
  4. FLASH Photonen-Strahlführungen und Optiken (FS-FLASH-B)
  5. FS-FLASH (FS-FLASH)
  6. Soft X-Ray Port (XFEL_E2_SXP)
Research Program(s):
  1. 632 - Materials – Quantum, Complex and Functional Materials (POF4-632) (POF4-632)
  2. 6G2 - FLASH (DESY) (POF4-6G2) (POF4-6G2)
  3. FS-Proposal: F-20200784 EC (F-20200784-EC) (F-20200784-EC)
  4. 05K22FK2 - Verbundprojekt 05K2022 - 10K-THz-k-ToF: 10K ToF-Impulsmikroskop für FLASH mit Terahertz Anregung und Raumladungsunterdrückung. Teilprojekt 2. (BMBF-05K22FK2) (BMBF-05K22FK2)
  5. SFB 925 B02 - Ultraschnelle Dynamik in stark korrelierten Systemen (B02) (201270818) (201270818)
  6. CALIPSOplus - Convenient Access to Light Sources Open to Innovation, Science and to the World (730872) (730872)
Experiment(s):
  1. FLASH Beamline PG2 (FLASH)

Appears in the scientific report 2024
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Private Collections > >DESY > >FS > FS-FLASH-O
Private Collections > >DESY > >FS > FS-FLASH
Private Collections > >DESY > >FS > FS-LA
Private Collections > >XFEL.EU > XFEL_E2_SXP
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 Record created 2024-08-20, last modified 2025-07-15


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