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@ARTICLE{Puntel:613152,
author = {Puntel, Denny and Kutnyakhov, Dmytro and Wenthaus, Lukas
and Scholz, Markus and Wind, Nils and Heber, Michael and
Brenner, Günter and Gu, Genda and Cava, Robert J. and
Bronsch, Wibke and Cilento, Federico and Parmigiani, Fulvio
and Pressacco, Federico},
title = {{O}ut-of-equilibrium charge redistribution in a
copper-oxide based superconductor by time-resolved {X}-ray
photoelectron spectroscopy},
journal = {Scientific reports},
volume = {14},
number = {1},
issn = {2045-2322},
address = {[London]},
publisher = {Macmillan Publishers Limited, part of Springer Nature},
reportid = {PUBDB-2024-05578},
pages = {8775},
year = {2024},
abstract = {Charge-transfer excitations are of paramount importance for
understanding the electronic structure of copper-oxide based
high-temperature superconductors. In this study, we
investigate the response of a $Bi_2Sr_2CaCu_2O_{8+\delta}$
crystal to the charge redistribution induced by an infrared
ultrashort pulse. Element-selective time-resolved core-level
photoelectron spectroscopy with a high energy resolution
allows disentangling the dynamics of oxygen ions with
different coordination and bonds thanks to their different
chemical shifts. Our experiment shows that the O 1s
component arising from the Cu–O planes is significantly
perturbed by the infrared light pulse. Conversely, the
apical oxygen, also coordinated with Sr ions in the Sr-O
planes, remains unaffected. This result highlights the
peculiar behavior of the electronic structure of the Cu–O
planes. It also unlocks the way to study the
out-of-equilibrium electronic structure of
copper-oxide-based high-temperature superconductors by
identifying the O 1s core-level emission originating from
the oxygen ions in the Cu–O planes. This ability could be
critical to gain information about the strongly-correlated
electron ultrafast dynamical mechanisms in the Cu–O plane
in the normal and superconducting phases.},
cin = {FS-LA / DOOR ; HAS-User / FS-FLASH-O / FS-FLASH-B /
FS-FLASH / $XFEL_E2_SXP$},
ddc = {600},
cid = {I:(DE-H253)FS-LA-20130416 / I:(DE-H253)HAS-User-20120731 /
I:(DE-H253)FS-FLASH-O-20160930 /
I:(DE-H253)FS-FLASH-B-20160930 /
I:(DE-H253)FS-FLASH-20140814 /
$I:(DE-H253)XFEL_E2_SXP-20240106$},
pnm = {632 - Materials – Quantum, Complex and Functional
Materials (POF4-632) / 6G2 - FLASH (DESY) (POF4-6G2) /
FS-Proposal: F-20200784 EC (F-20200784-EC) / 05K22FK2 -
Verbundprojekt 05K2022 - 10K-THz-k-ToF: 10K
ToF-Impulsmikroskop für FLASH mit Terahertz Anregung und
Raumladungsunterdrückung. Teilprojekt 2. (BMBF-05K22FK2) /
SFB 925 B02 - Ultraschnelle Dynamik in stark korrelierten
Systemen (B02) (201270818) / CALIPSOplus - Convenient Access
to Light Sources Open to Innovation, Science and to the
World (730872)},
pid = {G:(DE-HGF)POF4-632 / G:(DE-HGF)POF4-6G2 /
G:(DE-H253)F-20200784-EC / G:(DE-Ds200)BMBF-05K22FK2 /
G:(GEPRIS)201270818 / G:(EU-Grant)730872},
experiment = {EXP:(DE-H253)F-PG2-20150101},
typ = {PUB:(DE-HGF)16},
pubmed = {38627427},
UT = {WOS:001207590500018},
doi = {10.1038/s41598-024-56440-4},
url = {https://bib-pubdb1.desy.de/record/613152},
}