Journal Article PUBDB-2018-02722

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Photophysics of indole upon X-ray absorption

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2018
RSC Publ. Cambridge

Physical chemistry, chemical physics 20, 20205 - 20216 () [10.1039/C8CP00936H]
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Abstract: A photofragmentation study of gas-phase indole $(C_8H_7N)$ upon single-photon ionization at a photon energy of 420 eV is presented. Indole was primarily inner-shell ionized at its nitrogen and carbon 1s orbitals. Electrons and ions were measured in coincidence by means of velocity map imaging. The angular relationship between ionic fragments is discussed along with the possibility to use the angle-resolved coincidence detection to perform experiments on molecules that are strongly oriented in their recoil-frame. The coincident measurement of electrons and ions revealed fragmentation-pathway-dependent electron spectra, linking the structural fragmentation dynamics to different electronic excitations. Evidence for photoelectron-impact self-ionization was observed.

Classification:

Note: © the Owner Societies

Contributing Institute(s):
  1. CFEL-Coherent X-Ray Imaging (FS-CFEL-1)
  2. Controlled Molecule Imaging (FS-CFEL-CMI)
  3. beauftragt von UNI (UNI/CUI)
Research Program(s):
  1. 6211 - Extreme States of Matter: From Cold Ions to Hot Plasmas (POF3-621) (POF3-621)
  2. 6G3 - PETRA III (POF3-622) (POF3-622)
  3. CUI - Hamburger Zentrum für ultraschnelle Beobachtung (194651731) (194651731)
  4. MEDEA - Molecular Electron Dynamics investigated by IntensE Fields and Attosecond Pulses (641789) (641789)
  5. VH-VI-419 - Dynamic Pathways in Multidimensional Landscapes (VH-VI-419) (VH-VI-419)
  6. IVF - Impuls- und Vernetzungsfonds (IVF-20140101) (IVF-20140101)
Experiment(s):
  1. PETRA Beamline P04 (PETRA III)

Appears in the scientific report 2018
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Medline ; Embargoed OpenAccess ; Allianz-Lizenz / DFG ; ClosedAccess ; Current Contents - Physical, Chemical and Earth Sciences ; IF < 5 ; JCR ; NCBI Molecular Biology Database ; NationallizenzNationallizenz ; SCOPUS ; Science Citation Index ; Science Citation Index Expanded ; Thomson Reuters Master Journal List ; Web of Science Core Collection
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Private Collections > >DESY > >FS > FS-CFEL-CMI
Private Collections > >DESY > >FS > FS-CFEL-1
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 Record created 2018-07-30, last modified 2025-07-17


Published on 2018-07-18. Available in OpenAccess from 2019-07-18.:
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