TypAmountVATCurrencyShareStatusCost centre
APC2540.000.00USD100.00 %(Zahlung erfolgt)810 / 476151
Sum2540.000.00(see parts above)   
Total2540.00     
Journal Article PUBDB-2026-00937

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3D atomic structure determination with ultrashort-pulse MeV electron diffraction

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2026
[Verlag nicht ermittelbar] Chester

IUCrJ 13(3), 282 - 290 () [10.1107/S2052252526002782]
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Abstract: Understanding structure at the atomic scale is fundamental for understanding the functioning and the development of materials with improved properties. Compared to other probes providing atomic resolution, electrons offer the strongest interaction in combination with minimal radiation damage, which makes them an ideal tool for investigating very small and radiation-sensitive samples (Henderson, 1995). However, these benefits are often offset by the laborious preparation of nanometre-sized samples that are not visible under the light microscope, and the fact that experiments are largely restricted to ultra-high vacuum (Duyvesteyn et al., 2018; Gruene et al., 2021). Here, we report the successful implementation of MeV electron diffraction for ab initio 3D structure determination of the quasi 2D material muscovite and the quantum material 1T-TaS₂ at atomic resolution. By employing ultrashort electron pulses from the REGAE accelerator, we obtained high-quality diffraction datasets suitable for structural refinements based on dynamical scattering theory, enabling precise localization of even hydrogen atoms. The increased penetration depth of MeV electrons significantly expands the applicable thickness range of samples, overcoming previous restrictions associated with traditional electron diffraction. These findings establish MeV electron diffraction as a viable approach for investigating a broad range of materials, including nanostructures and radiation-sensitive compounds, and open up new opportunities for in-situ and time-resolved experiments (Chao et al., 2023; Filippetto et al., 2022).

Classification:

Contributing Institute(s):
  1. FS-CFEL-1 Fachgruppe BMX (FS-CFEL-1-BMX)
  2. Injektion (MIN)
  3. FS-CFEL-1 (Group Leader: Henry Chapman) (CFEL-I)
  4. Beschleunigerphysik (MPY)
  5. Scientific computing (FS-SC)
  6. Bereichsleitung Beschleuniger / Bereich Beschleuniger (M)
  7. Koordination des XFEL-Beschleunigers (MXL)
  8. FS-SXQM (FS-SXQM)
Research Program(s):
  1. 632 - Materials – Quantum, Complex and Functional Materials (POF4-632) (POF4-632)
  2. 6G3 - PETRA III (DESY) (POF4-6G3) (POF4-6G3)
  3. InternLabs-0011 - HIR3X - Helmholtz International Laboratory on Reliability, Repetition, Results at the most advanced X-ray Sources (2020_InternLabs-0011) (2020_InternLabs-0011)
  4. DFG project G:(GEPRIS)390715994 - EXC 2056: CUI: Tiefe Einblicke in Materie (390715994) (390715994)
Experiment(s):
  1. Relativistic Electron Gun for Atomic Exploration
  2. PETRA Beamline P11 (PETRA III)

Appears in the scientific report 2026
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Medline ; Creative Commons Attribution CC BY 4.0 ; DOAJ ; OpenAccess ; Article Processing Charges ; Clarivate Analytics Master Journal List ; Current Contents - Physical, Chemical and Earth Sciences ; DOAJ Seal ; Essential Science Indicators ; Fees ; IF < 5 ; JCR ; PubMed Central ; SCOPUS ; Science Citation Index Expanded ; Web of Science Core Collection
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The record appears in these collections:
Private Collections > >DESY > >M > >MPY > MPY
Private Collections > >CFEL > >FS-CFEL > FS-CFEL-1-BMX
Private Collections > >CFEL > >FS-CFEL > CFEL-I
Private Collections > >DESY > >FS > FS-SXQM
Private Collections > >DESY > >FS > FS-SC
Private Collections > >DESY > >M > MXL
Private Collections > >DESY > >M > MIN
Private Collections > >DESY > >M > M
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 Record created 2026-03-09, last modified 2026-05-04