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Controlled molecule injector for cold, dense, and pure molecular beams at the European x-ray free-electron laser
He, L.CFEL*Extern*XFEL.EU* ; Johny, M.CFEL*Extern*XFEL.EU* ; Kierspel, T.CSSB*DESY* ; Dlugolecki, K.CFEL*XFEL.EU*DESY* ; Bari, S.DESY* ; Boll, R.XFEL.EU* ; Bromberger, H.CFEL*XFEL.EU*DESY* ; coreno, m.Extern*XFEL.EU* ; De Fanis, A.XFEL.EU* ; Di Fraia, M.Extern* ; Erk, B.XFEL.EU*DESY* ; Gisselbrecht, M.Extern* ; Grychtol, P.XFEL.EU* ; Eng-Johnsson, P.Extern*XFEL.EU* ; Mazza, T.XFEL.EU* ; Onvlee, J.CFEL*Extern*XFEL.EU* ; Ovcharenko, Y.XFEL.EU* ; Petrovic, J.Extern*XFEL.EU*DESY* ; Rennhack, N.XFEL.EU* ; Rivas, D.XFEL.EU* ; Rudenko, A.Extern* ; Ruehl, E.Extern* ; Schwob, L.XFEL.EU*DESY* ; Simon, M.Extern* ; Trinter, F.Extern*XFEL.EU* ; Usenko, S.XFEL.EU* ; Wiese, J.CFEL*Extern*XFEL.EU* ; Meyer, M.XFEL.EU* ; Trippel, S. (Corresponding author)CFEL*XFEL.EU*DESY* ; Küpper, J. (Corresponding author)CFEL*XFEL.EU*DESY*
2024
American Institute of Physics
[Erscheinungsort nicht ermittelbar]
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Please use a persistent id in citations: doi:10.1063/5.0219086 doi:10.3204/PUBDB-2024-06982
Abstract: A permanently available molecular-beam injection setup for controlled molecules (COMO) was installed and commissioned at the small quantum systems (SQS) instrument at the European x-ray free-electron laser (EuXFEL). A b-type electrostatic deflector allows for pure state-, size-, and isomer-selected samples of polar molecules and clusters. The source provides a rotationally cold (T ≈ 1 K) and dense (ρ ≈ 108 cm−3) molecular beam with pulse durations up to 100 µs generated by a new version of the Even-Lavie valve. Here, a performance overview of the COMO setup is presented along with characterization experiments performed both with an optical laser at the Center for Free-Electron-Laser Science and with x rays at EuXFEL under burst-mode operation. COMO was designed to be attached to different instruments at the EuXFEL, in particular, the SQS and single particles, clusters, and biomolecules (SPB) instruments. This advanced controlled-molecules injection setup enables x-ray free-electron laser studies using highly defined samples with soft and hard x-ray FEL radiation for applications ranging from atomic, molecular, and cluster physics to elementary processes in chemistry and biology.
Note: Open Access
Contributing Institute(s):
- The European XFEL Users (XFEL-User)
- Biomoleküle in Gasphase (FS-BIG)
Research Program(s):
- 631 - Matter – Dynamics, Mechanisms and Control (POF4-631) (POF4-631)
- DFG project G:(GEPRIS)194651731 - EXC 1074: Hamburger Zentrum für ultraschnelle Beobachtung (CUI): Struktur, Dynamik und Kontrolle von Materie auf atomarer Skala (194651731) (194651731)
- DFG project G:(GEPRIS)390715994 - EXC 2056: CUI: Advanced Imaging of Matter (390715994) (390715994)
- MEDEA - Molecular Electron Dynamics investigated by IntensE Fields and Attosecond Pulses (641789) (641789)
- HIRS-0018 - Helmholtz-Lund International School - Intelligent instrumentation for exploring matter at different time and length scales (HELIOS) (2020_HIRS-0018) (2020_HIRS-0018)
- 05K22GUA - Verbundprojekt 05K2022 - 2021-05992 UDIET: Ultraschnelle Dynamik des intermolekularen Energietransfers: elementare Schritte in Aerosolen und Flüssigchemie (BMBF-05K22GUA) (BMBF-05K22GUA)
- DFG project G:(GEPRIS)509471550 - Dynamik photoionisations-induzierter Prozesse in laser-präparierten Molekülen in der Gasphase und der wässrigen Phase (509471550) (509471550)
Experiment(s):
- SQS: Small Quantum Systems (SASE3)
- SPB: Single Particles, clusters & Biomolecules (SASE1)
Appears in the scientific report
2024
Database coverage:
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; Clarivate Analytics Master Journal List ; Current Contents - Engineering, Computing and Technology ; Current Contents - Physical, Chemical and Earth Sciences ; Ebsco Academic Search ; Essential Science Indicators ; IF < 5 ; JCR ; National-Konsortium ; SCOPUS ; Science Citation Index Expanded ; Web of Science Core Collection