Journal Article

PUBDB-2021-03561

http://join2-wiki.gsi.de/foswiki/pub/Main/Artwork/join2_logo100x88.png Modulated crystal structure of the atypical charge density wave state of single-crystal Lu$_2$Ir$_3$Si$_5$

Ramakrishnan, S.* ; Schoenleber, A.* ; Bao, J.* ; Rekis, T.* ; Kotla, S. R.Extern** ; Schaller, A.Extern** ; van Smaalen, S. (Corresponding author)Extern** ; Noohinejad, L.DESY* ; Tolkiehn, M.DESY* ; Paulmann, C.Extern* ; Sangeetha, N. S. ; Pal, D. ; Thamizhavel, A. ; Ramakrishnan, S. (Corresponding author)

2021
Inst. Woodbury, NY

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Please use a persistent id in citations: doi:10.1103/PhysRevB.104.054116  doi:10.3204/PUBDB-2021-03561

Abstract: The three-dimensional charge density wave (CDW) compound Lu$_2$Ir$_3$Si$_5$ undergoes a first-order CDW phase transition at around 200 K. An atypical CDW state is found, that is characterized by an incommensurate CDW with q=[0.2499(3),0.4843(4),0.2386(2)] at 60 K, and a large orthorhombic-to-triclinic lattice distortion with β=91.945(2)∘. We present the modulated crystal structure of the incommensurate CDW state. Structural analysis shows that the CDW resides on the zigzag chains of iridium atoms along c. The structural distortions are completely similar between nonmagnetic Lu$_2$Ir$_3$Si$_5$ and previously studied isostructural magnetic Er$_2$Ir$_3$Si$_5$5 with the small differences explained by the different values of the atomic radii of Lu and Er. Such a similarity is unique to R$_2$Ir$_3$Si$_5$ (R=rareearth). It differs from, for example, the rare-earth CDW compounds R$_5$Ir$_4$Si$_{10}$ for which Lu$_5$Ir$_4$Si$_{10}$ and Er5Ir4Si10 possess entirely different CDW states. We argue that the mechanism of CDW formation, thus, is different for R$_2$Ir$_3$Si$_5$ and R$_5$Ir$_4$Si$_{10}$.

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Contributing Institute(s):

1. DOOR-User (DOOR ; HAS-User)
2. Universität Bayreuth (UBT)
3. PETRA-D (FS-PETRA-D)

Research Program(s):

1. 631 - Matter – Dynamics, Mechanisms and Control (POF4-631) (POF4-631)
2. 6G3 - PETRA III (DESY) (POF4-6G3) (POF4-6G3)
3. FS-Proposal: I-20190544 (I-20190544) (I-20190544)

Experiment(s):

1. PETRA Beamline P24 (PETRA III)

Appears in the scientific report 2021

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Database coverage:
; ; ; Clarivate Analytics Master Journal List ; Current Contents - Electronics and Telecommunications Collection ; Current Contents - Physical, Chemical and Earth Sciences ; Ebsco Academic Search ; Essential Science Indicators ; IF < 5 ; JCR ; SCOPUS ; Science Citation Index Expanded ; Web of Science Core Collection

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