| Home > Publications database > Evolution of field-induced metastable phases in the Shastry-Sutherland lattice magnet TmB 4 |
| Journal Article | PUBDB-2020-03066 |
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2020
Inst.
Woodbury, NY
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Please use a persistent id in citations: doi:10.1103/PhysRevB.102.060407 doi:10.3204/PUBDB-2020-03066
Abstract: The appearance of a plateau in the magnetization of a quantum spin system subject to continuously varying magnetic field invites the identification of a topological quantization. Indeed, the magnetization plateaus at 1/8 and 1/2 of saturation in TmB4 have been suggested to be intrinsic, resulting from such a topological quantization, or, alternatively, to be metastable phases. By means of neutron- and x-ray-scattering experiments and magnetization measurements, we show that the 1/8 plateau is metastable, arising because the spin dynamics are frozen below T≈4.5 K. Our experiments show that in this part of the phase diagram of TmB4, many long-ranged orders with different propagation vectors may appear and coexist, particularly as the applied field drives the system from one plateau to another. The magnetic structures accommodating a magnetization of ≈1/8 seem to be particularly favorable, but still only appear if the system has sufficient dynamics to reorganize into a superstructure as it is driven toward the expected plateau. This work demonstrates that TmB4 represents a model material for the study of slow dynamics, in and out of equilibrium.
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