Journal Article PUBDB-2020-03066

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Evolution of field-induced metastable phases in the Shastry-Sutherland lattice magnet TmB 4

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2020
Inst. Woodbury, NY

Physical review / B 102(6), 060407 () [10.1103/PhysRevB.102.060407]
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Abstract: The appearance of a plateau in the magnetization of a quantum spin system subject to continuously varying magnetic field invites the identification of a topological quantization. Indeed, the magnetization plateaus at 1/8 and 1/2 of saturation in TmB4 have been suggested to be intrinsic, resulting from such a topological quantization, or, alternatively, to be metastable phases. By means of neutron- and x-ray-scattering experiments and magnetization measurements, we show that the 1/8 plateau is metastable, arising because the spin dynamics are frozen below T≈4.5 K. Our experiments show that in this part of the phase diagram of TmB4, many long-ranged orders with different propagation vectors may appear and coexist, particularly as the applied field drives the system from one plateau to another. The magnetic structures accommodating a magnetization of ≈1/8 seem to be particularly favorable, but still only appear if the system has sufficient dynamics to reorganize into a superstructure as it is driven toward the expected plateau. This work demonstrates that TmB4 represents a model material for the study of slow dynamics, in and out of equilibrium.

Classification:

Contributing Institute(s):
  1. DOOR-User (DOOR ; HAS-User)
  2. Experimentebetreuung PETRA III (FS-PET-S)
Research Program(s):
  1. 6212 - Quantum Condensed Matter: Magnetism, Superconductivity (POF3-621) (POF3-621)
  2. 6G3 - PETRA III (POF3-622) (POF3-622)
Experiment(s):
  1. PETRA Beamline P09 (PETRA III)

Appears in the scientific report 2020
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 Record created 2020-08-21, last modified 2025-07-16


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