Journal Article PUBDB-2016-02824

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Exciton recombination in one-dimensional organic Mott insulators

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2015
APS College Park, Md.

Physical review / B 92(20), 201104 () [10.1103/PhysRevB.92.201104]
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Abstract: We present a theory for the recombination of (charged) holons and doublons in one-dimensional organic Mott insulators, which is responsible for the decay of the photoexcited state. Due to the charge-spin separation, the dominant mechanism for recombination at low density of charges involves a multiphonon emission. We show that a reasonable coupling to phonons is sufficient to explain the fast recombination observed by pump-probe experiments in ET−F$_2$TCNQ, whereby we can also account for the measured pressure dependence of the recombination rate.

Classification:

Contributing Institute(s):
  1. Forschungsgruppe für strukturelle Dynamik (MPSD)
Research Program(s):
  1. 899 - ohne Topic (POF3-899) (POF3-899)
Experiment(s):
  1. No specific instrument

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Medline ; American Physical Society Transfer of Copyright Agreement ; OpenAccess ; Current Contents - Physical, Chemical and Earth Sciences ; IF < 5 ; JCR ; NationallizenzNationallizenz ; SCOPUS ; Science Citation Index ; Science Citation Index Expanded ; Thomson Reuters Master Journal List ; Web of Science Core Collection
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 Record created 2016-08-09, last modified 2025-07-30


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