Journal Article

DESY-2014-03776

http://join2-wiki.gsi.de/foswiki/pub/Main/Artwork/join2_logo100x88.png Generation and structure of extremely large clusters in pulsed jets

Rupp, D. (Corresponding Author)Extern* ; Adolph, M.Extern* ; Flückiger, L.Extern* ; Gorkhover, T.Extern* ; Müller, J. P.Extern* ; Müller, M.Extern* ; Sauppe, M.Extern* ; Wolter, D.Extern* ; Schorb, S.Extern* ; Treusch, R.DESY* ; Bostedt, C.Extern* ; Moeller, T.Extern*

2014
American Institute of Physics Melville, NY

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Please use a persistent id in citations: doi:10.1063/1.4890323

Abstract: Extremely large xenon clusters with sizes exceeding the predictions of the Hagena scaling law by several orders of magnitude are shown to be produced in pulsed gas jets. The cluster sizes are determined using single-shot single-particle imaging experiments with short-wavelength light pulses from the free-electron laser in Hamburg (FLASH). Scanning the time delay between the pulsed cluster source and the intense femtosecond x-ray pulses first shows a main plateau with size distributions in line with the scaling laws, which is followed by an after-pulse of giant clusters. For the extremely large clusters with radii of several hundred nanometers the x-ray scattering patterns indicate a grainy substructure of the particles, suggesting that they grow by cluster coagulation.

Note: OA

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Contributing Institute(s):

1. DOOR-User (DOOR)
2. Experimentebetreuung FLASH (FS-FL)

Research Program(s):

1. FLASH Beamline BL2 (POF2-54G16) (POF2-54G16)
2. FLASH Beamline BL3 (POF2-54G16) (POF2-54G16)

Experiment(s):

1. FLASH Beamline BL2 (FLASH)
2. FLASH Beamline BL3 (FLASH)

Appears in the scientific report 2014

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Database coverage:
; ; ; Allianz-Lizenz / DFG ; Current Contents - Social and Behavioral Sciences ; JCR ; NCBI Molecular Biology Database ; Nationallizenz ; SCOPUS ; Science Citation Index ; Science Citation Index Expanded ; Thomson Reuters Master Journal List ; Web of Science Core Collection

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