TY  - JOUR
AU  - Rupp, Daniela
AU  - Adolph, Marcus
AU  - Flückiger, Leonie
AU  - Gorkhover, Tais
AU  - Müller, Jan Philippe
AU  - Müller, Maria
AU  - Sauppe, Mario
AU  - Wolter, David
AU  - Schorb, Sebastian
AU  - Treusch, Rolf
AU  - Bostedt, Christoph
AU  - Moeller, Thomas
TI  - Generation and structure of extremely large clusters in pulsed jets
JO  - The journal of chemical physics
VL  - 141
IS  - 4
SN  - 1089-7690
CY  - Melville, NY
PB  - American Institute of Physics
M1  - DESY-2014-03776
SP  - 044306
PY  - 2014
N1  - OA
AB  - Extremely large xenon clusters with sizes exceeding the predictions of the Hagena scaling law by several orders of magnitude are shown to be produced in pulsed gas jets. The cluster sizes are determined using single-shot single-particle imaging experiments with short-wavelength light pulses from the free-electron laser in Hamburg (FLASH). Scanning the time delay between the pulsed cluster source and the intense femtosecond x-ray pulses first shows a main plateau with size distributions in line with the scaling laws, which is followed by an after-pulse of giant clusters. For the extremely large clusters with radii of several hundred nanometers the x-ray scattering patterns indicate a grainy substructure of the particles, suggesting that they grow by cluster coagulation.
LB  - PUB:(DE-HGF)16
UR  - <Go to ISI:>//WOS:000340712200043
C6  - pmid:25084909
DO  - DOI:10.1063/1.4890323
UR  - https://bib-pubdb1.desy.de/record/172525
ER  -