Report/Journal Article PHPPUBDB-24010

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Ab initio and photoemission study of correlation effects in $SrRuO_3$ thin films

 ;  ;  ;  ;  ; DESY

2013
APS College Park, Md.

Physical review / B 87(3), 035106 () [10.1103/PhysRevB.87.035106]
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Report No.: DESY-D-I-20100305 EC.

Abstract: We present the experimental and theoretical study of correlation effects in epitaxial SrRuO$_3$ thin films. Experimentally, we have performed resonant ultraviolet photoemission spectroscopy (UPS) and angle-resolved hard x-ray photoemission spectroscopy (HAXPES) measurements. For resonant UPS, the two methods, Fano-profile fitting of constant initial state spectra and the energy distribution curves equidistant difference spectra, were used to extract Ru 4$d$ partial spectral weight (PSW) in the valence band. We find Ru 4$d$ PSW possessing a clearly pronounced coherent peak at the Fermi level together with angle-resolved HAXPES spectra demonstrating no difference in surface and bulk electronic structure. From comparison of experimental data with theoretical calculations done at density functional theory level, we conclude that SrRuO$_3$ is a weakly correlated material and electronic structure of it can be consistently described employing first-principles approaches.

Classification:

Note: (c) American Physical Society. Post referee fulltext in progress. Code P.

Contributing Institute(s):
  1. Experiments with synchrotron radiation (HASYLAB(-2012))
Research Program(s):
  1. DORIS Beamline E1 (POF2-54G13) (POF2-54G13)
  2. DORIS Beamline BW2 (POF2-54G13) (POF2-54G13)
Experiment(s):
  1. DORIS Beamline E1 (DORIS III)
  2. DORIS Beamline BW2 (DORIS III)

Appears in the scientific report 2013
Database coverage:
American Physical Society Transfer of Copyright Agreement ; OpenAccess ; No Author Disambiguation
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 Record created 2013-01-18, last modified 2025-07-30


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