Journal Article PHPPUBDB-17976

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Synthesized Light Transients

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2011

Science 334, 195 () [10.1126/science.1210268]
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Abstract: Manipulation of electron dynamics calls for electromagnetic forces that can be confined to and controlled over sub-femtosecond time intervals. Tailored transients of light fields can provide these forces. We report on the generation of subcycle field transients spanning the infrared, visible, and ultraviolet frequency regimes with a 1.5-octave three-channel optical field synthesizer and their attosecond sampling. To demonstrate applicability, we field-ionized krypton atoms within a single wave crest and launched a valence-shell electron wavepacket with a well-defined initial phase. Half-cycle field excitation and attosecond probing revealed fine details of atomic-scale electron motion, such as the instantaneous rate of tunneling, the initial charge distribution of a valence-shell wavepacket, the attosecond dynamic shift (instantaneous ac Stark shift) of its energy levels, and its few-femtosecond coherent oscillations.


Contributing Institute(s):
  1. Experiments with synchrotron radiation (HASYLAB(-2012))
  2. CFEL-Theory (FS-CFEL-3)
  3. Forschungsgruppe für strukturelle Dynamik (MPSD)
Research Program(s):
  1. 54x - Programm Forschung mit Photonen, Neutronen, Ionen - Topic unbekannt (POF2-54x) (POF2-54x)
Experiment(s):
  1. No specific instrument

Appears in the scientific report 2011
Database coverage:
Medline ; JCR ; No Author Disambiguation ; Thomson Reuters Master Journal List ; Web of Science Core Collection
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The record appears in these collections:
Private Collections > >DESY > >FS > HASYLAB(-2012)
Private Collections > >DESY > >FS > FS-CFEL-3
Document types > Articles > Journal Article
Private Collections > >MPG > MPSD
Public records
Publications database

 Record created 2012-09-19, last modified 2025-07-30



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