TY - JOUR AU - Wirth, Adrian AU - Hassan, M. T. AU - Grguras, Ivanka AU - Gagnon, J. AU - Moulet, A. AU - Luu, T. T. AU - Pabst, Stefan AU - Santra, Robin AU - Alahmed, Z. A. AU - Azzeer, A. M. AU - Yakovlev, V. S. AU - Pervak, V. AU - Krausz, F. AU - Goulielmakis, E. AU - DESY TI - Synthesized Light Transients JO - Science VL - 334 SN - 0036-8075 M1 - PHPPUBDB-17976 SP - 195 PY - 2011 AB - Manipulation of electron dynamics calls for electromagnetic forces that can be confined to and controlled over sub-femtosecond time intervals. Tailored transients of light fields can provide these forces. We report on the generation of subcycle field transients spanning the infrared, visible, and ultraviolet frequency regimes with a 1.5-octave three-channel optical field synthesizer and their attosecond sampling. To demonstrate applicability, we field-ionized krypton atoms within a single wave crest and launched a valence-shell electron wavepacket with a well-defined initial phase. Half-cycle field excitation and attosecond probing revealed fine details of atomic-scale electron motion, such as the instantaneous rate of tunneling, the initial charge distribution of a valence-shell wavepacket, the attosecond dynamic shift (instantaneous ac Stark shift) of its energy levels, and its few-femtosecond coherent oscillations. LB - PUB:(DE-HGF)16 C6 - pmid:21903778 UR - <Go to ISI:>//WOS:000295833600038 DO - DOI:10.1126/science.1210268 UR - https://bib-pubdb1.desy.de/record/94718 ER -