Journal Article PUBDB-2026-00712

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Cavity Controls Core-to-Core Resonant Inelastic X-Ray Scattering

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2026
APS College Park, Md.

Physical review letters 136(6), 063601 () [10.1103/z6xz-p7cm]
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Abstract: X-ray cavity quantum optics with inner-shell transitions has been limited by the spectral overlap between resonant and continuum states. Here, we report the first experimental demonstration of cavity-controlled core-to-core resonant inelastic x-ray scattering (RIXS). We suppress the absorption-edge effects by monitoring the RIXS profile, thereby resolving the resonant state from the overlapping continuum. We observe distinct cavity-induced energy shifts and cavity-enhanced decay rates in the 2⁒𝑝⁒3⁒𝑑RIXS spectra of WSi$_2$. These effects, manifesting as stretched or shifted profiles in the RIXS planes, enable novel spectroscopic applications via cavity-controlled core-hole states. Our results establish core-to-core RIXS as a powerful tool to manipulate inner-shell dynamics in x-ray cavities, offering new avenues for integrating quantum optical effects with x-ray spectroscopy.

Classification:

Contributing Institute(s):
  1. PETRA-D (FS-PETRA-D)
  2. FXE (XFEL_E1_FXE)
Research Program(s):
  1. 631 - Matter – Dynamics, Mechanisms and Control (POF4-631) (POF4-631)
  2. 6G3 - PETRA III (DESY) (POF4-6G3) (POF4-6G3)
  3. FS-Proposal: I-20220927 (I-20220927) (I-20220927)
Experiment(s):
  1. Measurement at external facility

Appears in the scientific report 2026
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Medline ; Creative Commons Attribution CC BY 4.0 ; OpenAccess ; Clarivate Analytics Master Journal List ; Current Contents - Electronics and Telecommunications Collection ; Current Contents - Physical, Chemical and Earth Sciences ; Ebsco Academic Search ; Essential Science Indicators ; IF >= 5 ; JCR ; NationallizenzNationallizenz ; SCOAP3 sponsored Journal ; SCOPUS ; Science Citation Index Expanded ; Web of Science Core Collection
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Private Collections > >XFEL.EU > XFEL_E1_FXE
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 Record created 2026-02-11, last modified 2026-02-13


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