Journal Article PUBDB-2024-07592

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Field-induced magnetic transitions in the highly anisotropic ferrimagnet ErFe$_5$Al$_7$ studied by high-field x-ray magnetic dichroism

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2024
Inst. Woodbury, NY

Physical review / B 109(9), 094404 () [10.1103/PhysRevB.109.094404]
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Abstract: We present a comprehensive study of the magnetic properties of the strongly anisotropic ferrimagnet ErFe$_5$Al$_7$ in pulsed magnetic fields up to 30 T applied along the hard magnetization axis within the basal plane of the tetragonal lattice around the compensation temperature (𝑇$_{comp}$). Macroscopic measurements showed two anomalies at about 8 T and 25 T in a small temperature range around 𝑇$_{comp}$. High-field x-ray magnetic circular dichroism (XMCD) data at the Er 𝑀5- and the Fe 𝐿3-edge resonances provide insight into the element-selective magnetization processes, revealing a coherent rotation of Er 4⁒𝑓 and Fe 3⁒𝑑 moments, with stepwise jumps including an unexpected one from an easy to a hard magnetization axis. XMCD at the Er 𝐿3-edge resonance elucidates the role of Er 5⁒𝑑 electrons in coupling the Er 4⁒𝑓 and the Fe 3⁒𝑑 moments. Finally, an in-plane anisotropy constant was evaluated from a simulation of the magnetization process at temperatures well below 𝑇$_{comp}$ using a two-sublattice model.

Classification:

Contributing Institute(s):
  1. FS-PS Fachgruppe HIBEF (FS-HIBEF)
  2. HED (XFEL_E1_HED)
Research Program(s):
  1. 631 - Matter – Dynamics, Mechanisms and Control (POF4-631) (POF4-631)
  2. DFG project G:(GEPRIS)247310070 - SFB 1143: Korrelierter Magnetismus: Von Frustration zu Topologie (247310070) (247310070)
  3. DFG project G:(GEPRIS)390858490 - EXC 2147: KomplexitΓ€t und Topologie in Quantenmaterialien (CT.QMAT) (390858490) (390858490)
Experiment(s):
  1. Measurement at external facility

Appears in the scientific report 2024
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 Record created 2024-12-12, last modified 2025-07-15


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