Journal Article PUBDB-2024-06674

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Fluorescence-mediated postcollision interaction in x-ray photoionization of the Xe K edge

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2024
Inst. Woodbury, NY

Physical review / A 110(2), 023117 () [10.1103/PhysRevA.110.023117]
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Abstract: Postcollision interaction (PCI) in near-threshold photoionization of the 𝐾 shell of atomic Xe is investigated with hard-x-ray synchrotron radiation. Applying Auger electron spectroscopy, line-shape distortion is monitored in the $𝐾−𝐿_2→𝐿_2⁢𝑀_{4,5}⁢𝑀_{4,5}$ decay channel, where the initial $𝐾−𝐿_2$ $(𝐾⁢𝛼_2)$ x-ray-emission step mediates the emission of the two continuum electrons. The 𝐾-edge result is compared to similar data obtained on direct $𝐿_2⁢𝑀_{4,5}⁢𝑀_{4,5}$ decay at the $𝐿_2$ edge without x-ray-emission. It is found that the evolution of the PCI shift with excess photon energy is very similar at both edges, but a subtle decrease in the PCI shift is observable at the 𝐾 edge due to the effect of the ultrafast x-ray emission step delaying the PCI energy exchange by a few attoseconds.

Classification:

Contributing Institute(s):
  1. CFEL-CMI (FS-CFEL-CMI)
  2. Uni Hamburg / Experimentalphysik (UNI/EXP)
Research Program(s):
  1. 631 - Matter – Dynamics, Mechanisms and Control (POF4-631) (POF4-631)
  2. DFG project G:(GEPRIS)255652344 - SPP 1840: Quantum Dynamics in Tailored Intense Fields (QUTIF) (255652344) (255652344)
Experiment(s):
  1. No specific instrument

Appears in the scientific report 2024
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 Record created 2024-11-12, last modified 2025-07-23


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