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| Journal Article | PUBDB-2023-03207 |
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2023
APS
College Park, Md.
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Please use a persistent id in citations: doi:10.1103/PhysRevLett.131.253201 doi:10.3204/PUBDB-2023-03207
Abstract: Excited double-core-hole states of isolated water molecules resulting from the sequential absorption oftwo x-ray photons have been investigated. These states are formed through an alternative pathway, wherethe initial step of core ionization is accompanied by the shake-up of a valence electron, leading to the samefinal states as in the core-ionization followed by core-excitation pathway. The capability of the x-rayfree-electron laser to deliver very intense, very short, and tunable light pulses is fully exploited to identifythe two different pathways.
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