Journal Article PUBDB-2020-05288

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Compact Ho:YLF-pumped ZnGeP$_{2}$ -based optical parametric amplifiers tunable in the molecular fingerprint regime

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2020
Soc. Washington, DC

Optics letters 45(8), 2255 () [10.1364/OL.389535]
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Abstract: We report on a compact mid-infrared laser architecture, comprising a chain of ZnGeP2-based optical parametric amplifiers (OPAs), which afford a higher energy yield (<∼60 µJ at 1 kHz) compared to most conventional OPA gain media transparent in the 2–8-µm wavelength range. Specifically, our OPA scheme allows ready tunability in the molecular fingerprint regime and is tailored for strong-field excitation and coherent control of both stretch and bend (or torsional) vibrational modes in molecules. The OPAs are pumped and directly seeded (via supercontinuum generation) by a 2-µm, 3-ps Ho:YLF regenerative amplifier. The compressibility of the OPA output is demonstrated by a representative measurement of the near-Gaussiantemporal profile of a dispersion-compensated 105-fs idler pulse at a central wavelength of 5.1 µm, corresponding to ∼6 optical cycles. Detailed numerical simulations closelycorroborate the experimental measurements, providing a benchmark and a platform to further explore the parameter space for future design, optimization, and implementation of high-energy, ultrafast, mid-infrared laser schemes.

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Contributing Institute(s):
  1. Laser Forschung und Entwicklung (FS-LA)
  2. MPSD (CFEL-SSUMP)
  3. MPSD (CFEL-ARD)
Research Program(s):
  1. 6211 - Extreme States of Matter: From Cold Ions to Hot Plasmas (POF3-621) (POF3-621)
Experiment(s):
  1. No specific instrument

Appears in the scientific report 2020
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 Record created 2020-12-27, last modified 2025-07-16


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