Home > Publications database > Compact Ho:YLF-pumped ZnGeP$_{2}$ -based optical parametric amplifiers tunable in the molecular fingerprint regime |
Journal Article | PUBDB-2020-05288 |
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2020
Soc.
Washington, DC
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Please use a persistent id in citations: doi:10.1364/OL.389535
Abstract: We report on a compact mid-infrared laser architecture, comprising a chain of ZnGeP2-based optical parametric amplifiers (OPAs), which afford a higher energy yield (<∼60 µJ at 1 kHz) compared to most conventional OPA gain media transparent in the 2–8-µm wavelength range. Specifically, our OPA scheme allows ready tunability in the molecular fingerprint regime and is tailored for strong-field excitation and coherent control of both stretch and bend (or torsional) vibrational modes in molecules. The OPAs are pumped and directly seeded (via supercontinuum generation) by a 2-µm, 3-ps Ho:YLF regenerative amplifier. The compressibility of the OPA output is demonstrated by a representative measurement of the near-Gaussiantemporal profile of a dispersion-compensated 105-fs idler pulse at a central wavelength of 5.1 µm, corresponding to ∼6 optical cycles. Detailed numerical simulations closelycorroborate the experimental measurements, providing a benchmark and a platform to further explore the parameter space for future design, optimization, and implementation of high-energy, ultrafast, mid-infrared laser schemes.
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