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000453490 1001_ $$0P:(DE-H253)PIP1031811$$aCheng, Siqi$$b0
000453490 245__ $$aCompact Ho:YLF-pumped ZnGeP$_{2}$ -based optical parametric amplifiers tunable in the molecular fingerprint regime
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000453490 520__ $$aWe report on a compact mid-infrared laser architecture, comprising a chain of ZnGeP2-based optical parametric amplifiers (OPAs), which afford a higher energy yield (<∼60 µJ at 1 kHz) compared to most conventional OPA gain media transparent in the 2–8-µm wavelength range. Specifically, our OPA scheme allows ready tunability in the molecular fingerprint regime and is tailored for strong-field excitation and coherent control of both stretch and bend (or torsional) vibrational modes in molecules. The OPAs are pumped and directly seeded (via supercontinuum generation) by a 2-µm, 3-ps Ho:YLF regenerative amplifier. The compressibility of the OPA output is demonstrated by a representative measurement of the near-Gaussiantemporal profile of a dispersion-compensated 105-fs idler pulse at a central wavelength of 5.1 µm, corresponding to ∼6 optical cycles. Detailed numerical simulations closelycorroborate the experimental measurements, providing a benchmark and a platform to further explore the parameter space for future design, optimization, and implementation of high-energy, ultrafast, mid-infrared laser schemes.
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000453490 7001_ $$0P:(DE-H253)PIP1024646$$aChatterjee, Gourab$$b1
000453490 7001_ $$0P:(DE-H253)PIP1007800$$aTellkamp, Friedjof$$b2
000453490 7001_ $$0P:(DE-H253)PIP1024674$$aLang, Tino$$b3
000453490 7001_ $$0P:(DE-H253)PIP1017957$$aRuehl, Axel$$b4
000453490 7001_ $$0P:(DE-H253)PIP1018794$$aHartl, Ingmar$$b5$$eCorresponding author
000453490 7001_ $$0P:(DE-HGF)0$$aDwayne Miller, R. J.$$b6$$eCorresponding author
000453490 773__ $$0PERI:(DE-600)1479014-2$$a10.1364/OL.389535$$gVol. 45, no. 8, p. 2255 -$$n8$$p2255$$tOptics letters$$v45$$x1539-4794$$y2020
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