Journal Article PUBDB-2018-04106

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Generation and characterization of ultrathin free-flowing liquid sheets

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2018
Springer Nature [London]

Nature Communications 9(1), 1353 () [10.1038/s41467-018-03696-w]
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Abstract: The physics and chemistry of liquid solutions play a central role in science, and our understanding of life on Earth. Unfortunately, key tools for interrogating aqueous systems, such as infrared and soft X-ray spectroscopy, cannot readily be applied because of strong absorption in water. Here we use gas-dynamic forces to generate free-flowing, sub-micron, liquid sheets which are two orders of magnitude thinner than anything previously reported. Optical, infrared, and X-ray spectroscopies are used to characterize the sheets, which are found to be tunable in thickness from over 1 μm down to less than 20 nm, which corresponds to fewer than 100 water molecules thick. At this thickness, aqueous sheets can readily transmit photons across the spectrum, leading to potentially transformative applications in infrared, X-ray, electron spectroscopies and beyond. The ultrathin sheets are stable for days in vacuum, and we demonstrate their use at free-electron laser and synchrotron light sources.

Classification:

Contributing Institute(s):
  1. DOOR-User (DOOR)
  2. FLASH Wissenschaftlicher Nutzerbetrieb (FS-FLASH-O)
  3. European XFEL Projekt Team (Eur.XFEL)
Research Program(s):
  1. 6211 - Extreme States of Matter: From Cold Ions to Hot Plasmas (POF3-621) (POF3-621)
  2. 6G2 - FLASH (POF3-622) (POF3-622)
Experiment(s):
  1. FLASH Beamline BL3 (FLASH)

Appears in the scientific report 2018
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Medline ; Creative Commons Attribution CC BY 4.0 ; DOAJ ; OpenAccess ; BIOSIS Previews ; Clarivate Analytics Master Journal List ; Current Contents - Agriculture, Biology and Environmental Sciences ; Current Contents - Life Sciences ; Current Contents - Physical, Chemical and Earth Sciences ; DOAJ Seal ; IF >= 10 ; JCR ; NCBI Molecular Biology Database ; PubMed Central ; SCOPUS ; Science Citation Index ; Science Citation Index Expanded ; Web of Science Core Collection ; Zoological Record
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Author Correction: Generation and characterization of ultrathin free-flowing liquid sheets ist
Nature Communications 9(1), 2860 () [10.1038/s41467-018-05365-4]  GO OpenAccess  Download fulltext Files BibTeX | EndNote: XML, Text | RIS

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Author Correction: Generation and characterization of ultrathin free-flowing liquid sheets
Nature Communications 10(1), 1615 () [10.1038/s41467-019-09457-7]  GO OpenAccess  Download fulltext Files BibTeX | EndNote: XML, Text | RIS


 Record created 2018-11-01, last modified 2025-07-17


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