Stimulated X-Ray Raman Scattering with Free-Electron Laser Sources

Rohringer, N.; Maxwell, T.; Bostedt, C.; Sanchez-Gonzalez, A.; Krzywinski, J.; Purvis, M.; Rubensson, J. E.; Agåker, M.; Lutman, A.; Nordgren, J.; Weninger, C.; Squibb, R.; Muecke, Oliver D.; Erk, B.; Zhaunerchyk, V.; Rocca, J. J.; Rolles, D.; Ilchen, M.; Såthe, C.; Kimberg, V.; Küpper, J.; Lindahl, A. O.; Ryan, D.; Mullins, T.; Coffee, R. N.; Carron Monterro, S.; London, R. A.; Kierspel, T.; Mucke, M.; Bozek, J. D.; Feifel, R.

doi:10.1007/978-3-319-19521-6_26

Contribution to a book

PUBDB-2016-06343

Stimulated X-Ray Raman Scattering with Free-Electron Laser Sources

Rohringer, N. (Corresponding author)CFEL*MPG* ; Kimberg, V. ; Weninger, C. ; Sanchez-Gonzalez, A. ; Lutman, A. ; Maxwell, T. ; Bostedt, C. ; Carron Monterro, S. ; Lindahl, A. O. ; Ilchen, M. ; Coffee, R. N. ; Bozek, J. D. ; Krzywinski, J. ; Kierspel, T.CFEL*DESY* ; Mullins, T.CFEL*DESY* ; Küpper, J.CFEL*DESY* ; Erk, B.DESY* ; Rolles, D.Extern* ; Muecke, O. D.CFEL*DESY* ; London, R. A. ; Purvis, M. ; Ryan, D. ; Rocca, J. J. ; Feifel, R. ; Squibb, R. ; Zhaunerchyk, V. ; Såthe, C. ; Agåker, M. ; Mucke, M. ; Nordgren, J. ; Rubensson, J. E.

2016
Springer International Publishing Cham
ISBN: 978-3-319-19520-9 (print), 978-3-319-19521-6 (electronic)

X-Ray Lasers 2014 Cham : Springer International Publishing, Springer Proceedings in Physics 169, 201 - 207 (2016) [10.1007/978-3-319-19521-6_26]

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Please use a persistent id in citations: doi:10.1007/978-3-319-19521-6_26

Abstract: Stimulated electronic x-ray Raman scattering is the building block for several proposed x-ray pump probe techniques, that would allow the study of electron dynamics at unprecedented timescales. We present high spectral resolution data on stimulated electronic x-ray Raman scattering in a gas sample of neon using a self-amplified spontaneous emission x-ray free-electron laser. Despite the limited spectral coherence and broad bandwidth of these sources, high-resolution spectra can be obtained by statistical methods, opening the path to coherent stimulated x-ray Raman spectroscopy. An extension of these ideas to molecules and the results of a recent experiment in CO are discussed.

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