Journal Article PUBDB-2016-02162

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Direct observation of half-metallicity in the Heusler compound $Co_{2}MnSi$

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2014
Nature Publishing Group London

Nature Communications 5, 3974 () [10.1038/ncomms4974]
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Abstract: Ferromagnetic thin films of Heusler compounds are highly relevant for spintronic applications owing to their predicted half-metallicity, that is, 100% spin polarization at the Fermi energy. However, experimental evidence for this property is scarce. Here we investigate epitaxial thin films of the compound Co2MnSi in situ by ultraviolet-photoemission spectroscopy, taking advantage of a novel multi-channel spin filter. By this surface sensitive method, an exceptionally large spin polarization of (93^{+7}_{-11}) % at room temperature is observed directly. As a more bulk sensitive method, additional ex situ spin-integrated high energy X-ray photoemission spectroscopy experiments are performed. All experimental results are compared with advanced band structure and photoemission calculations which include surface effects. Excellent agreement is obtained with calculations, which show a highly spin polarized bulk-like surface resonance ingrained in a half metallic bulk band structure.

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Contributing Institute(s):
  1. PETRA III Extension (FS-PEX)
Research Program(s):
  1. 6214 - Nanoscience and Materials for Information Technology (POF3-621) (POF3-621)
Experiment(s):
  1. PETRA Beamline P09 (PETRA III)

Appears in the scientific report 2014
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 Record created 2016-06-07, last modified 2025-07-17


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