Journal Article PUBDB-2016-00477

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Time-resolved studies with FELs

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2015
Elsevier New York, NY [u.a.]

Journal of electron spectroscopy and related phenomena 204, 228 - 236 () [10.1016/j.elspec.2015.07.010]
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Abstract: Intense femtosecond VUV, XUV, and X-ray pulses from free-electron lasers (FELs) enable time-resolved experiments studying ultrafast dynamics in a large variety of systems relevant, e.g., to physics, chemistry, biology, and material sciences. In this paper, we focus on time-resolved studies of gas-phase molecules, which lie at the crossroad between atomic, molecular and optical physics and ultrafast photochemistry. We describe the current status of the field and discuss typical experimental configurations used for pump-probe experiments with FELs. We illustrate them with three recent examples for such experiments performed at the FLASH and LCLS FELs studying charge transfer following XUV and X-ray photoabsorption as well as photoelectron diffraction from aligned molecules. We conclude with a short outlook on future developments and perspectives for femtosecond pump-probe experiments with FELs.

Classification:

Note: (c) Elsevier B.V. Post referee full text in progress (embargo 1 year from 30 July 2015).

Contributing Institute(s):
  1. Experimentebetreuung FLASH (FS-FL)
  2. DOOR-User (DOOR)
  3. Strukturdynamik Chemischer Systeme (FS-SCS)
Research Program(s):
  1. 6211 - Extreme States of Matter: From Cold Ions to Hot Plasmas (POF3-621) (POF3-621)
  2. 6G2 - FLASH (POF3-622) (POF3-622)
Experiment(s):
  1. FLASH Beamline BL2 (FLASH)
  2. FLASH Beamline BL3 (FLASH)

Appears in the scientific report 2015
Database coverage:
Medline ; Current Contents - Physical, Chemical and Earth Sciences ; IF < 5 ; JCR ; NationallizenzNationallizenz ; SCOPUS ; Science Citation Index ; Science Citation Index Expanded ; Thomson Reuters Master Journal List ; Web of Science Core Collection
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 Record created 2016-01-18, last modified 2025-07-17


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