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000643497 1001_ $$0P:(DE-H253)PIP1091875$$aHeighway, Patrick$$b0$$eCorresponding author
000643497 245__ $$aX-ray thermal diffuse scattering as a texture-robust temperature diagnostic for dynamically compressed solids
000643497 260__ $$aMelville, NY$$bAmerican Inst. of Physics$$c2025
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000643497 520__ $$aWe present a model of x-ray thermal diffuse scattering (TDS) from a cubic polycrystal with an arbitrary crystallographic texture, based on the classic approach of Warren [B. E. Warren, Acta Crystallogr. 6, 803 (1953)]. We compare the predictions of our model with femtosecond x-ray diffraction patterns gathered from ambient and dynamically compressed rolled copper foils obtained at the High Energy Density instrument of the European X-Ray Free-Electron Laser facility and find that the texture-aware TDS model yields more accurate results than does the conventional powder model owed to Warren. Nevertheless, we further show: with sufficient angular detector coverage, the TDS signal is largely unchanged by sample orientation and in all cases strongly resembles the signal from a perfectly random powder; shot-to-shot fluctuations in the TDS signal resulting from grain-sampling statistics are at the percent level, in stark contrast to the fluctuations in the Bragg-peak intensities (which are over an order of magnitude greater); and TDS is largely unchanged even following texture evolution caused by compression-induced plastic deformation. We conclude that TDS is robust against texture variation, making it a flexible temperature diagnostic applicable just as well to off-the-shelf commercial foils as to ideal powders.
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000643497 773__ $$0PERI:(DE-600)1476463-5$$a10.1063/5.0295250$$gVol. 138, no. 15, p. 155903$$n15$$p155903$$tJournal of applied physics$$v138$$x0021-8979$$y2025
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