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| Home > Publications database > Tailoring p-Type Behavior in ZnO Quantum Dots through Enhanced Sol–Gel Synthesis: Mechanistic Insights into Zinc Vacancies > print |
| 001 | 614554 | ||
| 005 | 20250723172355.0 | ||
| 024 | 7 | _ | |2 doi |a 10.1021/acs.jpclett.3c03519 |
| 024 | 7 | _ | |2 datacite_doi |a 10.3204/PUBDB-2024-05900 |
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| 037 | _ | _ | |a PUBDB-2024-05900 |
| 041 | _ | _ | |a English |
| 082 | _ | _ | |a 530 |
| 100 | 1 | _ | |a Kahraman, Abdullah |b 0 |
| 245 | _ | _ | |a Tailoring p-Type Behavior in ZnO Quantum Dots through Enhanced Sol–Gel Synthesis: Mechanistic Insights into Zinc Vacancies |
| 260 | _ | _ | |a Washington, DC |b ACS |c 2024 |
| 336 | 7 | _ | |2 DRIVER |a article |
| 336 | 7 | _ | |2 DataCite |a Output Types/Journal article |
| 336 | 7 | _ | |0 PUB:(DE-HGF)16 |2 PUB:(DE-HGF) |a Journal Article |b journal |m journal |s 1726230092_4159809 |
| 336 | 7 | _ | |2 BibTeX |a ARTICLE |
| 336 | 7 | _ | |2 ORCID |a JOURNAL_ARTICLE |
| 336 | 7 | _ | |0 0 |2 EndNote |a Journal Article |
| 520 | _ | _ | |a The synthesis and control of properties of p-type ZnO iscrucial for a variety of optoelectronic and spintronic applications;however, it remains challenging due to the control of intrinsic midgap(defect) states. In this study, we demonstrate a synthetic route to yieldcolloidal ZnO quantum dots (QD) via an enhanced sol−gel processthat effectively eliminates the residual intermediate reaction molecules,which would otherwise weaken the excitonic emission. This processsupports the creation of ZnO with p-type properties or compensationof inherited n-type defects, primarily due to zinc vacancies underoxygen-rich conditions. The in-depth analysis of carrier recombinationin the midgap across several time scales reveals microsecond carrierlifetimes at room temperature which are expected to occur via zinc vacancy defects, supporting the promoted p-type character of thesynthesized ZnO QDs. |
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| 542 | _ | _ | |i 2024-02-07 |2 Crossref |u https://creativecommons.org/licenses/by/4.0/ |
| 588 | _ | _ | |a Dataset connected to CrossRef, Journals: bib-pubdb1.desy.de |
| 693 | _ | _ | |0 EXP:(DE-H253)XFEL-Exp-20150101 |1 EXP:(DE-H253)XFEL-20150101 |5 EXP:(DE-H253)XFEL-Exp-20150101 |a XFEL |e Experiments at XFEL |x 0 |
| 700 | 1 | _ | |a Socie, Etienne |b 1 |
| 700 | 1 | _ | |0 0000-0002-0087-7334 |a Nazari, Maryam |b 2 |
| 700 | 1 | _ | |0 0000-0002-2124-2813 |a Kazazis, Dimitrios |b 3 |
| 700 | 1 | _ | |a Buldu-Akturk, Merve |b 4 |
| 700 | 1 | _ | |a Kabanova, Victoria |b 5 |
| 700 | 1 | _ | |a Biasin, Elisa |b 6 |
| 700 | 1 | _ | |a Smolentsev, Grigory |b 7 |
| 700 | 1 | _ | |a Grolimund, Daniel |b 8 |
| 700 | 1 | _ | |0 0000-0002-8395-0364 |a Erdem, Emre |b 9 |
| 700 | 1 | _ | |a Moser, Jacques E. |b 10 |
| 700 | 1 | _ | |a Cannizzo, Andrea |b 11 |
| 700 | 1 | _ | |0 P:(DE-H253)PIP1081422 |a Bacellar Cases da Silveira, Camila |b 12 |e Corresponding author |
| 700 | 1 | _ | |0 P:(DE-H253)PIP1018116 |a Milne, Christopher |b 13 |e Corresponding author |
| 773 | 1 | 8 | |a 10.1021/acs.jpclett.3c03519 |b American Chemical Society (ACS) |d 2024-02-07 |n 6 |p 1755-1764 |3 journal-article |2 Crossref |t The Journal of Physical Chemistry Letters |v 15 |y 2024 |x 1948-7185 |
| 773 | _ | _ | |a 10.1021/acs.jpclett.3c03519 |g Vol. 15, no. 6, p. 1755 - 1764 |0 PERI:(DE-600)2522838-9 |n 6 |p 1755-1764 |t The journal of physical chemistry letters |v 15 |y 2024 |x 1948-7185 |
| 856 | 4 | _ | |u https://bib-pubdb1.desy.de/record/614554/files/kahraman-et-al-2024-tailoring-p-type-behavior-in-zno-quantum-dots-through-enhanced-sol-gel-synthesis-mechanistic.pdf |y OpenAccess |
| 856 | 4 | _ | |u https://bib-pubdb1.desy.de/record/614554/files/kahraman-et-al-2024-tailoring-p-type-behavior-in-zno-quantum-dots-through-enhanced-sol-gel-synthesis-mechanistic.pdf?subformat=pdfa |x pdfa |y OpenAccess |
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