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Cut-Off Extension of High-Harmonic Generation in Neon by Non-Sinusoidal Sub-Cycle Optical Waveforms

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2024

Final AttoChem Workshop, AttoChem2024, La LagunaLa Laguna, Spain, 28 Feb 2024 - 1 Mar 20242024-02-282024-03-01 1 pp. ()  GO

Abstract: Extending the spectrum of attosecond pulses obtained via high-harmonic generation toward higher photon-energies is an important goal for attosecond spectroscopy.An extension of the cut-off photon energy of the high-harmonic spectrum is observed when the process is driven by non-sinusoidal waveforms with durations down to belowa single optical cycle. Specifically, while the phase-matched high-harmonic spectra generated in Neon by a "sinusoidal" pulse, with a wavelength of 1.6 μm and durationof 1.5 optical cycles, extends up to ~350 eV, the spectra driven by a non-sinusoidal pulse, with a central wavelength of 1.4 μm and duration down to 0.5 optical cycles,extends up to ~400 eV.This shows experimentally how non-sinusoidal sub-cycle waveforms violate the well known proportionality of the cut-off photon energy with the square of the central wavelength.


Contributing Institute(s):
  1. Ultrafast Lasers & X-rays Division (FS-CFEL-2)
Research Program(s):
  1. 631 - Matter – Dynamics, Mechanisms and Control (POF4-631) (POF4-631)
Experiment(s):
  1. Experiments at CFEL

Appears in the scientific report 2024
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 Record created 2024-05-15, last modified 2024-05-21


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