TY - JOUR
AU - Lever, Fabiano
AU - Picconi, David
AU - Mayer, Dennis
AU - Alisauskas, Skirmantas
AU - Calegari, Francesca
AU - Duesterer, Stefan
AU - Feifel, Raimund
AU - Kuhlmann, Marion
AU - Mazza, Tommaso
AU - Metje, Jan
AU - Robinson, Matthew
AU - Squibb, Richard
AU - Trabattoni, Andrea
AU - Ware, Matthew
AU - Saalfrank, Peter
AU - Wolf, Thomas
AU - Guehr, Markus
TI - Direct observation of ππ<sup>*</sup> to nπ<sup>*</sup> transition in 2-thiouracil via time resolved NEXAFS spectroscopy
JO - The journal of physical chemistry letters
VL - 16
SN - 1948-7185
CY - Washington, DC
PB - ACS
M1 - PUBDB-2024-01318
SP - 4038 - 4046
PY - 2025
AB - The photophysics of nucleobases has been the object of both theoretical and experimental studies over the past decades, due to the challenges posed by the non-BOA (Born-Oppenheimer Approximation) dynamics in their relaxation pathway. In this context, the ultrafast dynamics of 2-thiouracil has been investigated with a time-resolved NEXAFS study at the Free Electron Laser FLASH.We show that x-ray absorption spectroscopy can be used to observe electronic transitions in ultrafast molecular relaxation. We use a uv-pump / x-ray probe scheme to measure the changes induced by photoexcitation to the x-ray absorption at the sulfur 2s and 2p edges, identifying absorption features corresponding to the S2 (ππ*) and S1 (nπ*) electronic states. We observe a delay of 102 ± 11 fs in the population of the nπ* state with respect to the initial optical excitation. We furthermore identify the presence of coherent oscillations in the absorption signal that match a similar observation in our previous x-ray photoelectron spectroscopy study.
LB - PUB:(DE-HGF)16
C6 - 40232202
UR - <Go to ISI:>//WOS:001467403900001
DO - DOI:10.1021/acs.jpclett.5c00544
UR - https://bib-pubdb1.desy.de/record/605144
ER -