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000599842 1001_ $$0P:(DE-H253)PIP1099002$$aWalther, Alexandre$$b0
000599842 245__ $$aGuest-Induced Reversible Transformation between an Azulene-Based Pd$_2$L$_4$ Lantern-Shaped Cage and a Pd$_4$L$_8$ Tetrahedron
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000599842 520__ $$aAzulene,a bluestructuralisomerof naphthalene,isintroducedas the backbonefor a new familyof Pd(II)-basedself-assemblies.Threeorganicligands,equippedwithvaryingdonorgroups,producethree[Pd$_2$L$_4$] cagesof differentcavitydimensions.Unexpectedly,the additionof organicdisulfonategueststo thesmallestlantern-shapedcage(featuringpyridinedonors)led to arapidandquantitativetransformationto a distorted-tetrahedral[Pd4L8] species.On the contrary,[Pd$_2$L$_4$] cagesformedfromligandswithisoquinolinedonorseitherjust encapsulatedthe guestsorshowedno interaction.Thetetrahedralspeciescouldbe fullyrevertedbackto its original[Pd$_2$L$_4$] topologyby capturingthe guestby another,strongerbinding[Pd$_2$L´$_4$] coordinationcage,narcissis-ticallyself-sortingfromthe firstcage.Theazulenes,servingascoloredhydrocarbonbackbonesof minimalatomcount,allowone to followcage assemblyand guest-inducedtransformationby thenakedeye. Furthermore,we proposethat theirpeculiarelectronicstructureinfluencesthe system’sassemblybehavior.
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000599842 7001_ $$0P:(DE-H253)PIP1033519$$aRegeni, Irene$$b1
000599842 7001_ $$0P:(DE-H253)PIP1009920$$aHolstein, Julian J.$$b2
000599842 7001_ $$0P:(DE-H253)PIP1031561$$aClever, Guido$$b3$$eCorresponding author
000599842 773__ $$0PERI:(DE-600)1472210-0$$a10.1021/jacs.3c09295$$gVol. 145, no. 46, p. 25365 - 25371$$n46$$p25365 - 25371$$tJournal of the American Chemical Society$$v145$$x0002-7863$$y2023
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