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@ARTICLE{Holmes:482764,
author = {Holmes, Susannah and Kirkwood, Henry J. and Bean, Richard
and Giewekemeyer, Klaus and Martin, Andrew V. and
Hadian-Jazi, Marjan and Wiedorn, Max O. and Oberthür,
Dominik and Marman, Hugh and Adriano, Luigi and Al-Qudami,
Nasser and Bajt, Saša and Barák, Imrich and Bari, Sadia
and Bielecki, Johan and Brockhauser, Sandor and Coleman,
Mathew A. and Cruz-Mazo, Francisco and Danilevski, Cyril and
Dörner, Katerina and Gañán-Calvo, Alfonso M. and
Graceffa, Rita and Fanghor, Hans and Heymann, Michael and
Frank, Matthias and Kaukher, Alexander and Kim, Yoonhee and
Kobe, Bostjan and Knoška, Juraj and Laurus, Torsten and
Letrun, Romain and Maia, Luis and Messerschmidt, Marc and
Metz, Markus and Michelat, Thomas and Mills, Grant and
Molodtsov, Serguei and Monteiro, Diana C. F. and Morgan,
Andrew J. and Münnich, Astrid and Peña Murillo, Gisel E.
and Previtali, Gianpietro and Round, Adam and Sato, Tokushi
and Schubert, Robin and Schulz, Joachim and Shelby, Megan
and Seuring, Carolin and Sellberg, Jonas A. and Sikorski,
Marcin and Silenzi, Alessandro and Stern, Stephan and
Sztuk-Dambietz, Jola and Szuba, Janusz and Trebbin, Martin
and Vagovic, Patrick and Ve, Thomas and Weinhausen, Britta
and Wrona, Krzysztof and Xavier, Paul Lourdu and Xu, Chen
and Yefanov, Oleksandr and Nugent, Keith A. and Chapman,
Henry N. and Mancuso, Adrian P. and Barty, Anton and Abbey,
Brian and Darmanin, Connie},
title = {{M}egahertz pulse trains enable multi-hit serial
femtosecond crystallography experiments at {X}-ray free
electron lasers},
journal = {Nature Communications},
volume = {13},
number = {1},
issn = {2041-1723},
address = {[London]},
publisher = {Nature Publishing Group UK},
reportid = {PUBDB-2022-04937},
pages = {4708},
year = {2022},
abstract = {The European X-ray Free Electron Laser (XFEL) and Linac
Coherent Light Source (LCLS) II are extremely intense
sources of X-rays capable of generating Serial Femtosecond
Crystallography (SFX) data at megahertz (MHz) repetition
rates. Previous work has shown that it is possible to use
consecutive X-ray pulses to collect diffraction patterns
from individual crystals. Here, we exploit the MHz pulse
structure of the European XFEL to obtain two complete
datasets from the same lysozyme crystal, first hit and the
second hit, before it exits the beam. The two datasets,
separated by <1 µs, yield up to 2.1 Å resolution
structures. Comparisons between the two structures reveal no
indications of radiation damage or significant changes
within the active site, consistent with the calculated dose
estimates. This demonstrates MHz SFX can be used as a tool
for tracking sub-microsecond structural changes in
individual single crystals, a technique we refer to as
multi-hit SFX.},
cin = {FS-CFEL-1 / MPSD / FS-ML / FS-BIG / CSSB-CF-CRYO /
$XFEL_E1_SPB/SFX$},
ddc = {500},
cid = {I:(DE-H253)FS-CFEL-1-20120731 / I:(DE-H253)MPSD-20120731 /
I:(DE-H253)FS-ML-20120731 / I:(DE-H253)FS-BIG-20220318 /
I:(DE-H253)CSSB-CF-CRYO-20210520 /
$I:(DE-H253)XFEL_E1_SPB_SFX-20210408$},
pnm = {633 - Life Sciences – Building Blocks of Life: Structure
and Function (POF4-633) / DFG project 194651731 - EXC 1074:
Hamburger Zentrum für ultraschnelle Beobachtung (CUI):
Struktur, Dynamik und Kontrolle von Materie auf atomarer
Skala (194651731) / DFG project 390715994 - EXC 2056: CUI:
Advanced Imaging of Matter (390715994)},
pid = {G:(DE-HGF)POF4-633 / G:(GEPRIS)194651731 /
G:(GEPRIS)390715994},
experiment = {EXP:(DE-H253)XFEL-SASE1-20150101},
typ = {PUB:(DE-HGF)16},
pubmed = {pmid:35953469},
UT = {WOS:000840107100020},
doi = {10.1038/s41467-022-32434-6},
url = {https://bib-pubdb1.desy.de/record/482764},
}