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@ARTICLE{Thesing:437083,
author = {Thesing, Linda Vanessa and Yachmenev, Andrey and
González-Férez, Rosario and Küpper, Jochen},
title = {{T}he {E}ffect of {N}uclear-{Q}uadrupole {C}oupling in the
{L}aser-{I}nduced {A}lignment of {M}olecules},
journal = {The journal of physical chemistry / A A, Molecules,
spectroscopy, kinetics, environment $\&$ general theory},
volume = {124},
number = {11},
issn = {1520-5215},
address = {Washington, DC},
publisher = {Soc.},
reportid = {PUBDB-2020-01318},
pages = {2225 - 2230},
year = {2020},
abstract = {We present a theoretical study of the time-dependent laser
alignment of molecules taking into account the hyperfine
coupling due to nuclear-quadrupole interactions. The
coupling of nuclear spins to the overall angular momentum of
molecules significantly influences their rotational
dynamics. Here, we systematically analyze the impact of the
nuclear-quadrupole coupling on the rotational dynamics of
the linear and the asymmetric-top diiodobenzene molecule
induced by external laser fields. We explore different
regimes of pulse shapes and laser-pulse intensities and
detail under which conditions the quadrupole coupling cannot
be neglected in the description of the laser alignment of
molecules.},
cin = {FS-CFEL-1 / FS-CFEL-CMI / UNI/EXP / UNI/CUI},
ddc = {530},
cid = {I:(DE-H253)FS-CFEL-1-20120731 /
I:(DE-H253)FS-CFEL-CMI-20220405 /
$I:(DE-H253)UNI_EXP-20120731$ /
$I:(DE-H253)UNI_CUI-20121230$},
pnm = {6211 - Extreme States of Matter: From Cold Ions to Hot
Plasmas (POF3-621) / DFG project 255652344 - SPP 1840:
Quantum Dynamics in Tailored Intense Fields (QUTIF)
(255652344) / DFG project 390715994 - EXC 2056: CUI:
Advanced Imaging of Matter (390715994) / DFG project
194651731 - EXC 1074: Hamburger Zentrum für ultraschnelle
Beobachtung (CUI): Struktur, Dynamik und Kontrolle von
Materie auf atomarer Skala (194651731) / DFG project
281310165 - Abbildung chemischer Dynamik mittels
laserinduzierter Elektronenbeugung im
Molekülkoordinatensystem (281310165) / Ex-Net-0002-Phase2-3
- Advanced Imaging of Matter: Structure, Dynamics and
Control on the Atomic Scale - AIM
$(2018_Ex-Net-0002-Phase2-3)$},
pid = {G:(DE-HGF)POF3-6211 / G:(GEPRIS)255652344 /
G:(GEPRIS)390715994 / G:(GEPRIS)194651731 /
G:(GEPRIS)281310165 / $G:(DE-HGF)2018_Ex-Net-0002-Phase2-3$},
experiment = {EXP:(DE-MLZ)NOSPEC-20140101},
typ = {PUB:(DE-HGF)16},
pubmed = {pmid:32077290},
UT = {WOS:000526392700012},
doi = {10.1021/acs.jpca.9b11433},
url = {https://bib-pubdb1.desy.de/record/437083},
}