% IMPORTANT: The following is UTF-8 encoded.  This means that in the presence
% of non-ASCII characters, it will not work with BibTeX 0.99 or older.
% Instead, you should use an up-to-date BibTeX implementation like “bibtex8” or
% “biber”.

@ARTICLE{Dong:435393,
      author       = {Dong, Renhao and Sahabudeen, Hafeesudeen and Qi, Haoyuan
                      and Ballabio, Marco and Položij, Miroslav and Olthof,
                      Selina and Shivhare, Rishi and Jing, Yu and Park, Sangwook
                      and Liu, Kejun and Zhang, Tao and Ma, Ji and Rellinghaus,
                      Bernd and Mannsfeld, Stefan C. B. and Bonn, Mischa and
                      Cánovas, Enrique and Zheng, Zhikun and Kaiser, Ute and
                      Feng, Xinliang and Heine, Thomas},
      title        = {{H}ighly {C}rystalline and {S}emiconducting {I}mine-{B}ased
                      {T}wo-{D}imensional {P}olymers {E}nabled by {I}nterfacial
                      {S}ynthesis},
      journal      = {Angewandte Chemie / International edition International
                      edition},
      volume       = {59},
      number       = {15},
      issn         = {1433-7851},
      address      = {Weinheim},
      publisher    = {Wiley-VCH},
      reportid     = {PUBDB-2020-00627},
      pages        = {6028 - 6036},
      year         = {2020},
      abstract     = {Single‐layer and multi‐layer 2D polyimine films have
                      been achieved through interfacial synthesis methods.
                      However, it remains a great challenge to achieve the maximum
                      degree of crystallinity in the 2D polyimines, which largely
                      limits the long‐range transport properties. Here we employ
                      a surfactant‐monolayer‐assisted interfacial synthesis
                      (SMAIS) method for the successful preparation of porphyrin
                      and triazine containing polyimine‐based 2D polymer
                      (PI‐2DP) films with square and hexagonal lattices,
                      respectively. The synthetic PI‐2DP films are featured with
                      polycrystalline multilayers with tunable thickness from 6 to
                      200 nm and large crystalline domains (100–150 nm in
                      size). Intrigued by high crystallinity and the presence of
                      electroactive porphyrin moieties, the optoelectronic
                      properties of PI‐2DP are investigated by time‐resolved
                      terahertz spectroscopy. Typically, the porphyrin‐based
                      PI‐2DP 1 film exhibits a p‐type semiconductor behavior
                      with a band gap of 1.38 eV and hole mobility as high as
                      0.01 cm2 V−1 s−1, superior to the previously
                      reported polyimine based materials.},
      cin          = {DOOR ; HAS-User},
      ddc          = {540},
      cid          = {I:(DE-H253)HAS-User-20120731},
      pnm          = {6G3 - PETRA III (POF3-622)},
      pid          = {G:(DE-HGF)POF3-6G3},
      experiment   = {EXP:(DE-H253)P-P03-20150101},
      typ          = {PUB:(DE-HGF)16},
      pubmed       = {pmid:31943664},
      UT           = {WOS:000512827700001},
      doi          = {10.1002/anie.201915217},
      url          = {https://bib-pubdb1.desy.de/record/435393},
}