000435393 001__ 435393
000435393 005__ 20250729150058.0
000435393 0247_ $$2doi$$a10.1002/anie.201915217
000435393 0247_ $$2ISSN$$a0044-8249
000435393 0247_ $$2ISSN$$a0570-0833
000435393 0247_ $$2ISSN$$a1433-7851
000435393 0247_ $$2ISSN$$a1521-3757
000435393 0247_ $$2ISSN$$a1521-3773
000435393 0247_ $$2datacite_doi$$a10.3204/PUBDB-2020-00627
000435393 0247_ $$2altmetric$$aaltmetric:76025422
000435393 0247_ $$2pmid$$apmid:31943664
000435393 0247_ $$2WOS$$aWOS:000512827700001
000435393 0247_ $$2openalex$$aopenalex:W2999992026
000435393 037__ $$aPUBDB-2020-00627
000435393 041__ $$aEnglish
000435393 082__ $$a540
000435393 1001_ $$0P:(DE-HGF)0$$aDong, Renhao$$b0$$eCorresponding author
000435393 245__ $$aHighly Crystalline and Semiconducting Imine-Based Two-Dimensional Polymers Enabled by Interfacial Synthesis
000435393 260__ $$aWeinheim$$bWiley-VCH$$c2020
000435393 3367_ $$2DRIVER$$aarticle
000435393 3367_ $$2DataCite$$aOutput Types/Journal article
000435393 3367_ $$0PUB:(DE-HGF)16$$2PUB:(DE-HGF)$$aJournal Article$$bjournal$$mjournal$$s1585735196_30609
000435393 3367_ $$2BibTeX$$aARTICLE
000435393 3367_ $$2ORCID$$aJOURNAL_ARTICLE
000435393 3367_ $$00$$2EndNote$$aJournal Article
000435393 520__ $$aSingle‐layer and multi‐layer 2D polyimine films have been achieved through interfacial synthesis methods. However, it remains a great challenge to achieve the maximum degree of crystallinity in the 2D polyimines, which largely limits the long‐range transport properties. Here we employ a surfactant‐monolayer‐assisted interfacial synthesis (SMAIS) method for the successful preparation of porphyrin and triazine containing polyimine‐based 2D polymer (PI‐2DP) films with square and hexagonal lattices, respectively. The synthetic PI‐2DP films are featured with polycrystalline multilayers with tunable thickness from 6 to 200 nm and large crystalline domains (100–150 nm in size). Intrigued by high crystallinity and the presence of electroactive porphyrin moieties, the optoelectronic properties of PI‐2DP are investigated by time‐resolved terahertz spectroscopy. Typically, the porphyrin‐based PI‐2DP 1 film exhibits a p‐type semiconductor behavior with a band gap of 1.38 eV and hole mobility as high as 0.01 cm2 V−1 s−1, superior to the previously reported polyimine based materials.
000435393 536__ $$0G:(DE-HGF)POF3-6G3$$a6G3 - PETRA III (POF3-622)$$cPOF3-622$$fPOF III$$x0
000435393 588__ $$aDataset connected to CrossRef
000435393 693__ $$0EXP:(DE-H253)P-P03-20150101$$1EXP:(DE-H253)PETRAIII-20150101$$6EXP:(DE-H253)P-P03-20150101$$aPETRA III$$fPETRA Beamline P03$$x0
000435393 7001_ $$0P:(DE-H253)PIP1081762$$aSahabudeen, Hafeesudeen$$b1
000435393 7001_ $$0P:(DE-HGF)0$$aQi, Haoyuan$$b2
000435393 7001_ $$0P:(DE-HGF)0$$aBallabio, Marco$$b3
000435393 7001_ $$0P:(DE-HGF)0$$aPoložij, Miroslav$$b4
000435393 7001_ $$0P:(DE-H253)PIP1010705$$aOlthof, Selina$$b5
000435393 7001_ $$0P:(DE-H253)PIP1029040$$aShivhare, Rishi$$b6
000435393 7001_ $$0P:(DE-HGF)0$$aJing, Yu$$b7
000435393 7001_ $$0P:(DE-H253)PIP1081861$$aPark, Sangwook$$b8
000435393 7001_ $$0P:(DE-H253)PIP1017772$$aLiu, Kejun$$b9
000435393 7001_ $$0P:(DE-HGF)0$$aZhang, Tao$$b10
000435393 7001_ $$0P:(DE-H253)PIP1085667$$aMa, Ji$$b11
000435393 7001_ $$0P:(DE-HGF)0$$aRellinghaus, Bernd$$b12
000435393 7001_ $$0P:(DE-H253)PIP1029114$$aMannsfeld, Stefan C. B.$$b13
000435393 7001_ $$0P:(DE-HGF)0$$aBonn, Mischa$$b14
000435393 7001_ $$0P:(DE-HGF)0$$aCánovas, Enrique$$b15
000435393 7001_ $$0P:(DE-HGF)0$$aZheng, Zhikun$$b16
000435393 7001_ $$0P:(DE-HGF)0$$aKaiser, Ute$$b17
000435393 7001_ $$0P:(DE-H253)PIP1081776$$aFeng, Xinliang$$b18$$eCorresponding author
000435393 7001_ $$0P:(DE-HGF)0$$aHeine, Thomas$$b19
000435393 773__ $$0PERI:(DE-600)2011836-3$$a10.1002/anie.201915217$$gVol. 59, no. 15, p. 6028 - 6036$$n15$$p6028 - 6036$$tAngewandte Chemie / International edition International edition$$v59$$x1433-7851$$y2020
000435393 8564_ $$uhttps://bib-pubdb1.desy.de/record/435393/files/anie.201915217.pdf$$yOpenAccess
000435393 8564_ $$uhttps://bib-pubdb1.desy.de/record/435393/files/anie.201915217.gif?subformat=icon$$xicon$$yOpenAccess
000435393 8564_ $$uhttps://bib-pubdb1.desy.de/record/435393/files/anie.201915217.jpg?subformat=icon-1440$$xicon-1440$$yOpenAccess
000435393 8564_ $$uhttps://bib-pubdb1.desy.de/record/435393/files/anie.201915217.jpg?subformat=icon-180$$xicon-180$$yOpenAccess
000435393 8564_ $$uhttps://bib-pubdb1.desy.de/record/435393/files/anie.201915217.jpg?subformat=icon-640$$xicon-640$$yOpenAccess
000435393 8564_ $$uhttps://bib-pubdb1.desy.de/record/435393/files/anie.201915217.pdf?subformat=pdfa$$xpdfa$$yOpenAccess
000435393 909CO $$ooai:bib-pubdb1.desy.de:435393$$pdnbdelivery$$pdriver$$pVDB$$popen_access$$popenaire
000435393 9101_ $$0I:(DE-HGF)0$$6P:(DE-H253)PIP1081762$$aExternal Institute$$b1$$kExtern
000435393 9101_ $$0I:(DE-HGF)0$$6P:(DE-H253)PIP1010705$$aExternal Institute$$b5$$kExtern
000435393 9101_ $$0I:(DE-HGF)0$$6P:(DE-H253)PIP1029040$$aExternal Institute$$b6$$kExtern
000435393 9101_ $$0I:(DE-HGF)0$$6P:(DE-H253)PIP1081861$$aExternal Institute$$b8$$kExtern
000435393 9101_ $$0I:(DE-HGF)0$$6P:(DE-H253)PIP1017772$$aExternal Institute$$b9$$kExtern
000435393 9101_ $$0I:(DE-HGF)0$$6P:(DE-H253)PIP1085667$$aExternal Institute$$b11$$kExtern
000435393 9101_ $$0I:(DE-HGF)0$$6P:(DE-H253)PIP1029114$$aExternal Institute$$b13$$kExtern
000435393 9101_ $$0I:(DE-HGF)0$$6P:(DE-H253)PIP1081776$$aExternal Institute$$b18$$kExtern
000435393 9131_ $$0G:(DE-HGF)POF3-622$$1G:(DE-HGF)POF3-620$$2G:(DE-HGF)POF3-600$$3G:(DE-HGF)POF3$$4G:(DE-HGF)POF$$9G:(DE-HGF)POF3-6G3$$aDE-HGF$$bForschungsbereich Materie$$lVon Materie zu Materialien und Leben$$vFacility topic: Research on Matter with Brilliant Light Sources$$x0
000435393 9141_ $$y2020
000435393 915__ $$0StatID:(DE-HGF)0200$$2StatID$$aDBCoverage$$bSCOPUS
000435393 915__ $$0LIC:(DE-HGF)CCBYNC4$$2HGFVOC$$aCreative Commons Attribution-NonCommercial CC BY-NC 4.0
000435393 915__ $$0StatID:(DE-HGF)1030$$2StatID$$aDBCoverage$$bCurrent Contents - Life Sciences
000435393 915__ $$0StatID:(DE-HGF)0600$$2StatID$$aDBCoverage$$bEbsco Academic Search
000435393 915__ $$0StatID:(DE-HGF)0100$$2StatID$$aJCR$$bANGEW CHEM INT EDIT : 2017
000435393 915__ $$0StatID:(DE-HGF)9910$$2StatID$$aIF >= 10$$bANGEW CHEM INT EDIT : 2017
000435393 915__ $$0StatID:(DE-HGF)0150$$2StatID$$aDBCoverage$$bWeb of Science Core Collection
000435393 915__ $$0StatID:(DE-HGF)0110$$2StatID$$aWoS$$bScience Citation Index
000435393 915__ $$0StatID:(DE-HGF)0111$$2StatID$$aWoS$$bScience Citation Index Expanded
000435393 915__ $$0StatID:(DE-HGF)0510$$2StatID$$aOpenAccess
000435393 915__ $$0StatID:(DE-HGF)0030$$2StatID$$aPeer Review$$bASC
000435393 915__ $$0StatID:(DE-HGF)1150$$2StatID$$aDBCoverage$$bCurrent Contents - Physical, Chemical and Earth Sciences
000435393 915__ $$0StatID:(DE-HGF)0310$$2StatID$$aDBCoverage$$bNCBI Molecular Biology Database
000435393 915__ $$0StatID:(DE-HGF)0300$$2StatID$$aDBCoverage$$bMedline
000435393 915__ $$0StatID:(DE-HGF)0420$$2StatID$$aNationallizenz
000435393 915__ $$0StatID:(DE-HGF)0199$$2StatID$$aDBCoverage$$bClarivate Analytics Master Journal List
000435393 9201_ $$0I:(DE-H253)HAS-User-20120731$$kDOOR ; HAS-User$$lDOOR-User$$x0
000435393 980__ $$ajournal
000435393 980__ $$aVDB
000435393 980__ $$aUNRESTRICTED
000435393 980__ $$aI:(DE-H253)HAS-User-20120731
000435393 9801_ $$aFullTexts