000423185 001__ 423185 000423185 005__ 20250716154042.0 000423185 0247_ $$2doi$$a10.1103/PhysRevApplied.11.064036 000423185 0247_ $$2datacite_doi$$a10.3204/PUBDB-2019-02481 000423185 0247_ $$2WOS$$aWOS:000471995300004 000423185 0247_ $$2altmetric$$aaltmetric:35719753 000423185 0247_ $$2arXiv$$aarXiv:1803.07472 000423185 0247_ $$2openalex$$aopenalex:W3105366809 000423185 037__ $$aPUBDB-2019-02481 000423185 041__ $$aEnglish 000423185 082__ $$a530 000423185 088__ $$2arXiv$$aarXiv:1803.07472 000423185 1001_ $$0P:(DE-H253)PIP1015352$$aLi, Zheng$$b0 000423185 245__ $$aAcoustic Funnel and Buncher for Nanoparticle Injection 000423185 260__ $$aCollege Park, Md. [u.a.]$$bAmerican Physical Society$$c2019 000423185 3367_ $$2DRIVER$$aarticle 000423185 3367_ $$2DataCite$$aOutput Types/Journal article 000423185 3367_ $$0PUB:(DE-HGF)16$$2PUB:(DE-HGF)$$aJournal Article$$bjournal$$mjournal$$s1720598776_1887848 000423185 3367_ $$2BibTeX$$aARTICLE 000423185 3367_ $$2ORCID$$aJOURNAL_ARTICLE 000423185 3367_ $$00$$2EndNote$$aJournal Article 000423185 520__ $$aAcoustics-based techniques are investigated to focus and bunch nanoparticle beams. This process allowsus to overcome the prominent problem of the longitudinal and transverse mismatch of particle-stream andx-ray-beam size in single-particle and single-molecule imaging at x-ray free-electron lasers (XFELs). Italso enables synchronized injection of particle streams at kilohertz repetition rates. Transverse focusingconcentrates the particle flux to the size of the (sub)micrometer X-ray focus. In the longitudinal direction,focused acoustic waves can be used to bunch the particle to the same repetition rate as the x-ray pulses.The acoustic manipulation is based on simple mechanical recoil effects and could be advantageous overlight-pressure-based methods, which rely on absorption. The acoustic equipment is easy to implement andcan be conveniently inserted into current XFEL endstations. With the proposed method, data collectiontimes could be reduced by a factor of $10^4$. This work does not just provide an efficient method for acousticmanipulation of streams of arbitrary gas-phase particles, but also opens up wide avenues for acousticsbasedparticle optics. 000423185 536__ $$0G:(DE-HGF)POF3-6211$$a6211 - Extreme States of Matter: From Cold Ions to Hot Plasmas (POF3-621)$$cPOF3-621$$fPOF III$$x0 000423185 536__ $$0G:(DE-HGF)POF3-6G13$$a6G13 - XFEL (POF3-622)$$cPOF3-622$$fPOF III$$x1 000423185 536__ $$0G:(DE-HGF)POF3-6G2$$a6G2 - FLASH (POF3-622)$$cPOF3-622$$fPOF III$$x2 000423185 536__ $$0G:(GEPRIS)194651731$$aDFG project 194651731 - EXC 1074: Hamburger Zentrum für ultraschnelle Beobachtung (CUI): Struktur, Dynamik und Kontrolle von Materie auf atomarer Skala (194651731)$$c194651731$$x3 000423185 536__ $$0G:(GEPRIS)390715994$$aDFG project 390715994 - EXC 2056: CUI: Advanced Imaging of Matter (390715994)$$c390715994$$x4 000423185 536__ $$0G:(DE-HGF)2018_Ex-Net-0002-Phase2-3$$aEx-Net-0002-Phase2-3 - Advanced Imaging of Matter: Structure, Dynamics and Control on the Atomic Scale - 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