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@ARTICLE{Amini:398834,
      author       = {Amini, Kasra and Savelyev, Evgeny and Brauße, Felix and
                      Berrah, Nora and Bomme, Cedric and Brouard, Mark and Burt,
                      Michael and Christensen, Lauge and Düsterer, Stefan and
                      Erk, Benjamin and Höppner, Hauke and Kierspel, Thomas and
                      Krecinic, Faruk and Lauer, Alexandra and Lee, Jason W. L.
                      and Müller, Maria and Mueller, Erland and Mullins, Terence
                      and Redlin, Harald and Schirmel, Nora and Thøgersen, Jan
                      and Techert, Simone and Toleikis, Sven and Treusch, Rolf and
                      Trippel, Sebastian and Ulmer, Anatoli and Vallance, Claire
                      and Wiese, Joss and Johnsson, Per and Küpper, Jochen and
                      Rudenko, Artem and Rouzée, Arnaud and Stapelfeldt, Henrik
                      and Rolles, Daniel and Boll, Rebecca},
      title        = {{P}hotodissociation of {A}ligned $\mathrm{{CH}_3{I}}$ and
                      $\mathrm{{C}_{6}{H}_{3}{F}_{2}{I}}$ {M}olecules {P}robed
                      with {T}ime-{R}esolved {C}oulomb {E}xplosion {I}maging by
                      {S}ite-{S}elective {XUV} {I}onization},
      journal      = {Structural dynamics},
      volume       = {5},
      number       = {1},
      issn         = {2329-7778},
      address      = {Melville, NY},
      publisher    = {AIP Publishing LLC},
      reportid     = {PUBDB-2018-00199},
      pages        = {014301 -},
      year         = {2018},
      abstract     = {We explore time-resolved Coulomb explosion induced by
                      intense, extreme ultraviolet (XUV) femtosecond pulses from a
                      free-electron laser as a method to image photo-induced
                      molecular dynamics in two molecules, iodomethane and
                      2,6-difluoroiodobenzene. At an excitation wavelength of
                      267 nm, the dominant reaction pathway in both molecules is
                      neutral dissociation via cleavage of the carbon–iodine
                      bond. This allows investigating the influence of the
                      molecular environment on the absorption of an intense,
                      femtosecond XUV pulse and the subsequent Coulomb explosion
                      process. We find that the XUV probe pulse induces local
                      inner-shell ionization of atomic iodine in dissociating
                      iodomethane, in contrast to non-selective ionization of all
                      photofragments in difluoroiodobenzene. The results reveal
                      evidence of electron transfer from methyl and phenyl
                      moieties to a multiply charged iodine ion. In addition,
                      indications for ultrafast charge rearrangement on the phenyl
                      radical are found, suggesting that time-resolved Coulomb
                      explosion imaging is sensitive to the localization of charge
                      in extended molecules.},
      cin          = {FS-SCS / FS-CFEL-CMI / FS-FLASH-D / FS-FLASH-O / Eur.XFEL},
      ddc          = {530},
      cid          = {I:(DE-H253)FS-SCS-20131031 /
                      I:(DE-H253)FS-CFEL-CMI-20220405 /
                      I:(DE-H253)FS-FLASH-D-20160930 /
                      I:(DE-H253)FS-FLASH-O-20160930 /
                      $I:(DE-H253)Eur_XFEL-20120731$},
      pnm          = {6211 - Extreme States of Matter: From Cold Ions to Hot
                      Plasmas (POF3-621) / 6G2 - FLASH (POF3-622) / ICONIC -
                      Imaging and CONtrol In Chemistry - ICONIC (238671) / MEDEA -
                      Molecular Electron Dynamics investigated by IntensE Fields
                      and Attosecond Pulses (641789) / CUI - Hamburger Zentrum
                      für ultraschnelle Beobachtung (194651731) / SFB 755 B03 -
                      Untersuchung ultraschneller Dynamik chemischer Reaktionen
                      mit Femtosekunden-Röntgenpulsen (B03) (50499717) / COMOTION
                      - Controlling the Motion of Complex Molecules and Particles
                      (614507)},
      pid          = {G:(DE-HGF)POF3-6211 / G:(DE-HGF)POF3-6G2 /
                      G:(EU-Grant)238671 / G:(EU-Grant)641789 /
                      G:(GEPRIS)194651731 / G:(GEPRIS)50499717 /
                      G:(EU-Grant)614507},
      experiment   = {EXP:(DE-H253)F-BL3-20150101},
      typ          = {PUB:(DE-HGF)16},
      pubmed       = {pmid:29430482},
      UT           = {WOS:000426844700001},
      doi          = {10.1063/1.4998648},
      url          = {https://bib-pubdb1.desy.de/record/398834},
}