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| 001 | 315807 | ||
| 005 | 20250730111440.0 | ||
| 024 | 7 | _ | |a 10.1088/1367-2630/18/10/103011 |2 doi |
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| 100 | 1 | _ | |a Kunnus, Kristjan |b 0 |
| 245 | _ | _ | |a Anti-Stokes resonant x-ray Raman scattering for atom specific and excited state selective dynamics |
| 260 | _ | _ | |a [Bad Honnef] |c 2016 |b Dt. Physikalische Ges. |
| 336 | 7 | _ | |a article |2 DRIVER |
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| 520 | _ | _ | |a Ultrafast electronic and structural dynamics of matter govern rate and selectivity of chemical reactions, as well as phase transitions and efficient switching in functional materials. Since x-rays determine electronic and structural properties with elemental, chemical, orbital and magnetic selectivity, short pulse x-ray sources have become central enablers of ultrafast science. Despite of these strengths, ultrafast x-rays have been poor at picking up excited state moieties from the unexcited ones. With time-resolved anti-Stokes resonant x-ray Raman scattering (AS-RXRS) performed at the LCLS, and ab initio theory we establish background free excited state selectivity in addition to the elemental, chemical, orbital and magnetic selectivity of x-rays. This unparalleled selectivity extracts low concentration excited state species along the pathway of photo induced ligand exchange of Fe(CO)$_5$ in ethanol. Conceptually a full theoretical treatment of all accessible insights to excited state dynamics with AS-RXRS with transform-limited x-ray pulses is given—which will be covered experimentally by upcoming transform-limited x-ray sources. |
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| 700 | 1 | _ | |a Josefsson, Ida |b 1 |
| 700 | 1 | _ | |a Rajkovic, Ivan |b 2 |
| 700 | 1 | _ | |a Schreck, Simon |b 3 |
| 700 | 1 | _ | |a Quevedo, Wilson |b 4 |
| 700 | 1 | _ | |a Beye, Martin |0 P:(DE-H253)PIP1005334 |b 5 |u desy |
| 700 | 1 | _ | |a Grübel, Sebastian |b 6 |
| 700 | 1 | _ | |a Scholz, Mirko |0 P:(DE-H253)PIP1007695 |b 7 |
| 700 | 1 | _ | |a Nordlund, Dennis |b 8 |
| 700 | 1 | _ | |a Zhang, Wenkai |b 9 |
| 700 | 1 | _ | |a Hartsock, Robert W |b 10 |
| 700 | 1 | _ | |a Gaffney, Kelly J |b 11 |
| 700 | 1 | _ | |a Schlotter, William F |b 12 |
| 700 | 1 | _ | |a Turner, Joshua J |b 13 |
| 700 | 1 | _ | |a Kennedy, Brian |b 14 |
| 700 | 1 | _ | |a Hennies, Franz |b 15 |
| 700 | 1 | _ | |a Techert, Simone |0 P:(DE-H253)PIP1008775 |b 16 |u desy |
| 700 | 1 | _ | |a Wernet, Philippe |b 17 |
| 700 | 1 | _ | |a Odelius, Michael |b 18 |
| 700 | 1 | _ | |a Föhlisch, Alexander |0 P:(DE-H253)PIP1002525 |b 19 |e Corresponding author |
| 773 | _ | _ | |a 10.1088/1367-2630/18/10/103011 |g Vol. 18, no. 10, p. 103011 - |0 PERI:(DE-600)1464444-7 |n 10 |p 103011 |t New journal of physics |v 18 |y 2016 |x 1367-2630 |
| 856 | 4 | _ | |u https://bib-pubdb1.desy.de/record/315807/files/Kunnus_2016_New_J._Phys._18_103011.pdf |y OpenAccess |
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