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@ARTICLE{Kunnus:315807,
      author       = {Kunnus, Kristjan and Josefsson, Ida and Rajkovic, Ivan and
                      Schreck, Simon and Quevedo, Wilson and Beye, Martin and
                      Grübel, Sebastian and Scholz, Mirko and Nordlund, Dennis
                      and Zhang, Wenkai and Hartsock, Robert W and Gaffney, Kelly
                      J and Schlotter, William F and Turner, Joshua J and Kennedy,
                      Brian and Hennies, Franz and Techert, Simone and Wernet,
                      Philippe and Odelius, Michael and Föhlisch, Alexander},
      title        = {{A}nti-{S}tokes resonant x-ray {R}aman scattering for atom
                      specific and excited state selective dynamics},
      journal      = {New journal of physics},
      volume       = {18},
      number       = {10},
      issn         = {1367-2630},
      address      = {[Bad Honnef]},
      publisher    = {Dt. Physikalische Ges.},
      reportid     = {PUBDB-2016-06076},
      pages        = {103011},
      year         = {2016},
      abstract     = {Ultrafast electronic and structural dynamics of matter
                      govern rate and selectivity of chemical reactions, as well
                      as phase transitions and efficient switching in functional
                      materials. Since x-rays determine electronic and structural
                      properties with elemental, chemical, orbital and magnetic
                      selectivity, short pulse x-ray sources have become central
                      enablers of ultrafast science. Despite of these strengths,
                      ultrafast x-rays have been poor at picking up excited state
                      moieties from the unexcited ones. With time-resolved
                      anti-Stokes resonant x-ray Raman scattering (AS-RXRS)
                      performed at the LCLS, and ab initio theory we establish
                      background free excited state selectivity in addition to the
                      elemental, chemical, orbital and magnetic selectivity of
                      x-rays. This unparalleled selectivity extracts low
                      concentration excited state species along the pathway of
                      photo induced ligand exchange of Fe(CO)$_5$ in ethanol.
                      Conceptually a full theoretical treatment of all accessible
                      insights to excited state dynamics with AS-RXRS with
                      transform-limited x-ray pulses is given—which will be
                      covered experimentally by upcoming transform-limited x-ray
                      sources.},
      cin          = {FS-SCS / FS-FLASH},
      ddc          = {530},
      cid          = {I:(DE-H253)FS-SCS-20131031 / I:(DE-H253)FS-FLASH-20140814},
      pnm          = {6215 - Soft Matter, Health and Life Sciences (POF3-621) /
                      DFG project 28586557 - SFB 755: Photonische Abbildungen auf
                      der Nanometerskala (28586557) / DFG project 217133147 - SFB
                      1073: Kontrolle von Energiewandlung auf atomaren Skalen
                      (217133147)},
      pid          = {G:(DE-HGF)POF3-6215 / G:(GEPRIS)28586557 /
                      G:(GEPRIS)217133147},
      experiment   = {EXP:(DE-MLZ)External-20140101},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:000386047000005},
      doi          = {10.1088/1367-2630/18/10/103011},
      url          = {https://bib-pubdb1.desy.de/record/315807},
}