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000315807 1001_ $$aKunnus, Kristjan$$b0
000315807 245__ $$aAnti-Stokes resonant x-ray Raman scattering for atom specific and excited state selective dynamics
000315807 260__ $$a[Bad Honnef]$$bDt. Physikalische Ges.$$c2016
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000315807 520__ $$aUltrafast electronic and structural dynamics of matter govern rate and selectivity of chemical reactions, as well as phase transitions and efficient switching in functional materials. Since x-rays determine electronic and structural properties with elemental, chemical, orbital and magnetic selectivity, short pulse x-ray sources have become central enablers of ultrafast science. Despite of these strengths, ultrafast x-rays have been poor at picking up excited state moieties from the unexcited ones. With time-resolved anti-Stokes resonant x-ray Raman scattering (AS-RXRS) performed at the LCLS, and ab initio theory we establish background free excited state selectivity in addition to the elemental, chemical, orbital and magnetic selectivity of x-rays. This unparalleled selectivity extracts low concentration excited state species along the pathway of photo induced ligand exchange of Fe(CO)$_5$ in ethanol. Conceptually a full theoretical treatment of all accessible insights to excited state dynamics with AS-RXRS with transform-limited x-ray pulses is given—which will be covered experimentally by upcoming transform-limited x-ray sources.
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000315807 536__ $$0G:(GEPRIS)217133147$$aDFG project 217133147 - SFB 1073: Kontrolle von Energiewandlung auf atomaren Skalen (217133147)$$c217133147$$x2
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000315807 7001_ $$aJosefsson, Ida$$b1
000315807 7001_ $$aRajkovic, Ivan$$b2
000315807 7001_ $$aSchreck, Simon$$b3
000315807 7001_ $$aQuevedo, Wilson$$b4
000315807 7001_ $$0P:(DE-H253)PIP1005334$$aBeye, Martin$$b5$$udesy
000315807 7001_ $$aGrübel, Sebastian$$b6
000315807 7001_ $$0P:(DE-H253)PIP1007695$$aScholz, Mirko$$b7
000315807 7001_ $$aNordlund, Dennis$$b8
000315807 7001_ $$aZhang, Wenkai$$b9
000315807 7001_ $$aHartsock, Robert W$$b10
000315807 7001_ $$aGaffney, Kelly J$$b11
000315807 7001_ $$aSchlotter, William F$$b12
000315807 7001_ $$aTurner, Joshua J$$b13
000315807 7001_ $$aKennedy, Brian$$b14
000315807 7001_ $$aHennies, Franz$$b15
000315807 7001_ $$0P:(DE-H253)PIP1008775$$aTechert, Simone$$b16$$udesy
000315807 7001_ $$aWernet, Philippe$$b17
000315807 7001_ $$aOdelius, Michael$$b18
000315807 7001_ $$0P:(DE-H253)PIP1002525$$aFöhlisch, Alexander$$b19$$eCorresponding author
000315807 773__ $$0PERI:(DE-600)1464444-7$$a10.1088/1367-2630/18/10/103011$$gVol. 18, no. 10, p. 103011 -$$n10$$p103011 $$tNew journal of physics$$v18$$x1367-2630$$y2016
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000315807 9141_ $$y2016
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