TY - JOUR AU - Priya, R. AU - Biukovic, G. AU - Manimekalai, M. AU - Lim, J. AU - Rao, S. S. AU - Grueber, G. AU - DESY TI - Solution structure of subunit (γ (γ1-204)) of the Mycobacterium tuberculosis F-ATP synthase and the unique loop of (γ165-178), representing a novel TB drug target JO - Journal of bioenergetics and biomembranes VL - 45 SN - 0145-479X CY - Dordrecht [u.a.] PB - Springer Science + Business Media B.V M1 - PHPPUBDB-25512 SP - 1-9 PY - 2013 N1 - © Springer Science+Business Media New York; Post referee fulltext in progress; Embargo 12 months from publication AB - Tuberculosis, caused by the strain Mycobacterium tuberculosis, is in focus of interest due to the emergence of multi- and extensive drug-resistant TB strains. The F(1)F(O) ATP synthase is one of the essential enzymes in energy requirement of both proliferating aerobic and hypoxic dormant stage of mycobacterium life cycle, and therefore a potential TB drug target. Subunit γ of F-ATP synthases plays an important role in coupling and catalysis via conformational transitions of its N- and C-termini as well as the bottom segment of the globular domain of γ, which is in close proximity to the rotating and ion-pumping c-ring. Here we describe the first production, purification and low resolution solution structure of subunit γ (γ(1-204), Mtγ(1-204)) of the M. tuberculosis F-ATP synthase. Mtγ(1-204) is a pear-like shaped protein with a molecular weight of 23 ± 2 kDa. Protein sequence analysis of Mtγ revealed differences in the amino acid composition to γ subunits from other sources, in particular the presence of a unique stretch of 13 amino acid residues (Mtγ(165-178)). NMR studies showed that Mtγ(165-178) forms a loop of polar residues. Mtγ(165-178) has been aligned at the bottom of the globular domain of the Escherichia coli subunit γ, being in close vicinity to the polar residues R41, Q42, E44 and Q46 (M. tuberculosis nomenclature) of the c-ring. The putative role(s) of Mtγ(165-178) in coupling and as a potential drug target are discussed. KW - Antitubercular Agents: chemistry KW - Antitubercular Agents: therapeutic use KW - Bacterial Proteins: antagonists & inhibitors KW - Bacterial Proteins: chemistry KW - Bacterial Proteins: genetics KW - Bacterial Proteins: metabolism KW - Catalysis KW - Drug Delivery Systems KW - Enzyme Inhibitors: chemistry KW - Enzyme Inhibitors: therapeutic use KW - Mycobacterium tuberculosis: enzymology KW - Mycobacterium tuberculosis: genetics KW - Nuclear Magnetic Resonance, Biomolecular KW - Protein Structure, Secondary KW - Protein Subunits: antagonists & inhibitors KW - Protein Subunits: chemistry KW - Protein Subunits: diagnostic use KW - Protein Subunits: metabolism KW - Proton-Translocating ATPases: antagonists & inhibitors KW - Proton-Translocating ATPases: chemistry KW - Proton-Translocating ATPases: genetics KW - Proton-Translocating ATPases: metabolism KW - Recombinant Proteins: antagonists & inhibitors KW - Recombinant Proteins: chemistry KW - Recombinant Proteins: genetics KW - Recombinant Proteins: metabolism KW - Tuberculosis: drug therapy KW - Tuberculosis: enzymology KW - Antitubercular Agents (NLM Chemicals) KW - Bacterial Proteins (NLM Chemicals) KW - Enzyme Inhibitors (NLM Chemicals) KW - Protein Subunits (NLM Chemicals) KW - Recombinant Proteins (NLM Chemicals) KW - Proton-Translocating ATPases (NLM Chemicals) LB - PUB:(DE-HGF)16 C6 - pmid:23104121 UR - <Go to ISI:>//WOS:000314899500011 DO - DOI:10.1007/s10863-012-9486-4 UR - https://bib-pubdb1.desy.de/record/142572 ER -