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@ARTICLE{Haikarainen:97456,
author = {Haikarainen, T. and Papageorgiou, A. C. and Tsoub, C.-C.
and Wub, J.-J. and DESY},
title = {{S}tructural characterization and biological implications
of di-zinc binding in the ferroxidase center of
{S}treptococcus pyogenes {D}pr.},
journal = {Biochemical and biophysical research communications},
volume = {398},
issn = {0006-291X},
address = {Orlando, Fla.},
publisher = {Academic Press},
reportid = {PHPPUBDB-20419},
pages = {361-365},
year = {2010},
abstract = {Dps proteins contain a ferroxidase site that binds and
oxidizes iron, thereby preventing hydroxyl radical formation
by Fenton reaction. Although the involvement of a di-iron
ferroxidase site has been suggested, X-ray crystal
structures of various Dps members have shown either one or
two iron cations with various occupancies despite the high
structural conservation of the site. Similarly, structural
studies with zinc, a redox-stable replacement for iron, have
shown the binding of either one or two zinc ions. Here, the
crystal structure of Streptococcus pyogenes Dpr in complex
with zinc reveals the binding of two zinc cations in the
ferroxidase center and an additional zinc-binding site at
the surface of the protein. The results suggest a structural
basis for the protection of Streptococcus pyogenes in zinc
stress conditions and provide a clear evidence for a di-zinc
and di-iron ferroxidase site in Streptococcus pyogenes Dpr
protein.},
keywords = {Bacterial Proteins: chemistry / Bacterial Proteins:
genetics / Binding Sites / Ceruloplasmin: chemistry /
Ceruloplasmin: genetics / Crystallography, X-Ray /
DNA-Binding Proteins: chemistry / DNA-Binding Proteins:
genetics / Protein Conformation / Streptococcus pyogenes:
enzymology / Zinc: chemistry / Bacterial Proteins (NLM
Chemicals) / DNA-Binding Proteins (NLM Chemicals) / Dpr
protein, Streptococcus (NLM Chemicals) / Zinc (NLM
Chemicals) / Ceruloplasmin (NLM Chemicals)},
cin = {EMBL},
ddc = {570},
cid = {$I:(DE-H253)EMBL_-2012_-20130307$},
pnm = {DORIS Beamline K1.2 (POF2-54G13)},
pid = {G:(DE-H253)POF2-K1.2-20130405},
experiment = {EXP:(DE-H253)D-K1.2-20150101},
typ = {PUB:(DE-HGF)16},
pubmed = {pmid:20599728},
UT = {WOS:000280867400005},
doi = {10.1016/j.bbrc.2010.06.071},
url = {https://bib-pubdb1.desy.de/record/97456},
}