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@ARTICLE{Linda:78396,
author = {Linda, O. C. and Salbu, B. and Janssens, K. and Proost, K.
and Dahlgaard, H. and DESY},
title = {{C}haracterization of uranium and plutonium containing
particles originating from the nuclear weapons accident in
{T}hule, {G}reenland, 1968},
journal = {Journal of environmental radioactivity},
volume = {81},
issn = {0265-931X},
address = {New York, NY [u.a.]},
publisher = {Elsevier},
reportid = {PHPPUBDB-3342},
pages = {32},
year = {2005},
abstract = {To improve long-term radioecological impact assessment for
the contaminated ecosystem of Bylot Sound, Greenland, U and
Pu containing particles have been characterized with respect
to particle size, elemental distribution, morphology and
oxidation states. Based on scanning electron microscopy with
XRMA, particles ranging from about 20 to 40 microm were
isolated. XRMA and mu-XRF mapping demonstrated that U and Pu
were homogeneously distributed throughout the particles,
indicating that U and Pu have been fused. Furthermore,
mu-XANES showed that U and Pu in the particles were present
as mixed oxides. U was found to be in oxidation state IV
whereas Pu apparently is a mixture of Pu(III) and Pu(IV). As
previous assessments are based on PuO2 only, revisions
should be made, taking Pu(III) into account.},
keywords = {Accidents, Aviation: statistics $\&$ numerical data /
Autoradiography / Electron Probe Microanalysis / Elementary
Particle Interactions / Geologic Sediments: analysis /
Greenland / Humans / Microscopy, Electron, Scanning /
Oxidation-Reduction / Particle Size / Plutonium: analysis /
Plutonium: chemistry / Radiation Monitoring: methods /
Radioactive Fallout: analysis / Radioactive Hazard Release:
statistics $\&$ numerical data / Soil Pollutants,
Radioactive: analysis / Spectrometry, Gamma / Synchrotrons /
Uranium: analysis / Uranium: chemistry / Water Pollutants,
Radioactive: analysis / Radioactive Fallout (NLM Chemicals)
/ Soil Pollutants, Radioactive (NLM Chemicals) / Water
Pollutants, Radioactive (NLM Chemicals) / Plutonium (NLM
Chemicals) / Uranium (NLM Chemicals)},
cin = {HASYLAB},
ddc = {690},
cid = {$I:(DE-H253)HASYLAB_-2012_-20130307$},
pnm = {DORIS Beamline L (POF1-550)},
pid = {G:(DE-H253)POF1-L-20130405},
experiment = {EXP:(DE-H253)D-L-20150101},
typ = {PUB:(DE-HGF)16},
pubmed = {pmid:15748658},
UT = {WOS:000228714500003},
doi = {10.1016/j.jenvrad.2004.10.013},
url = {https://bib-pubdb1.desy.de/record/78396},
}