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@ARTICLE{Trinter:646074,
author = {Trinter, Florian and Hofierka, Jaroslav and Rist, Jonas and
Kircher, Max and Weller, Miriam and Melzer, Niklas and
Tsitsonis, Dimitrios and Geyer, Angelina and Kruse, Jan and
Kastirke, Gregor and Williams, Joshua and Miteva, Tsveta and
Doerner, Reinhard and Schoeffler, Markus and Kunitski,
Maksim and SISOURAT, Nicolas and Cederbaum, Lorenz and
Jahnke, Till},
title = {{T}racking the {C}omplex {D}ynamics of
{E}lectron-{T}ransfer-{M}ediated {D}ecay in {R}eal {S}pace
and {T}ime},
journal = {Journal of the American Chemical Society},
volume = {148},
number = {4},
issn = {0002-7863},
address = {Washington, DC},
publisher = {ACS Publications},
reportid = {PUBDB-2026-00714},
pages = {4126 - 4135},
year = {2026},
note = {Open Access},
abstract = {When an electronically excited atom or molecule is embedded
in a chemical environment as, e.g., in a liquid or a loosely
bound cluster, it can de-excite through mechanisms where
neighboring atoms or molecules are actively participating in
the decay: either by donating or accepting energy or
electrons. For such nonlocal decay channels, nuclear
dynamics play a crucial role as they have a direct impact on
the decay efficiency itself. Here, we present a detailed
study of the electron-transfer-mediated decay in a loosely
bound triatomic prototype system, combining experimental
results from a 5-fold coincidence measurement and
theoretical modeling of the decay process. Depending on the
decay time, we find that certain classes of molecular
geometries are favored for this type of decay. Our findings
provide an intuitive picture of how
electron-transfer-mediated decay proceeds. In particular,
our results confirm a roaming-like behavior of the atoms of
the trimer prior to its decay. Our combined theoretical and
experimental approach enables a comprehensive tracing of the
real-space properties of the decaying system in the time
domain.},
cin = {DOOR ; HAS-User},
ddc = {540},
cid = {I:(DE-H253)HAS-User-20120731},
pnm = {6G3 - PETRA III (DESY) (POF4-6G3) / FS-Proposal: I-20191330
EC (I-20191330-EC) / DFG project G:(GEPRIS)509471550 -
Dynamik photoionisations-induzierter Prozesse in
laser-präparierten Molekülen in der Gasphase und der
wässrigen Phase (509471550) / $ETMD_ICEC$ - Efficient
pathways to neutralization and radical production enabled by
environment (692657)},
pid = {G:(DE-HGF)POF4-6G3 / G:(DE-H253)I-20191330-EC /
G:(GEPRIS)509471550 / G:(EU-Grant)692657},
experiment = {EXP:(DE-H253)P-P04-20150101},
typ = {PUB:(DE-HGF)16},
doi = {10.1021/jacs.5c15510},
url = {https://bib-pubdb1.desy.de/record/646074},
}