TY - JOUR
AU - Ganesan, A.
AU - Banerjee, Sourav
AU - Baral, S.
AU - Jose, J.
AU - Deshmukh, P. C.
AU - Manson, S. T.
TI - Relaxation effects in the photoionization time delay near the 3 s Cooper minimum of Ar
JO - Physical review / A
VL - 111
IS - 5
SN - 2469-9926
CY - Woodbury, NY
PB - Inst.
M1 - PUBDB-2026-00707
SP - 052805
PY - 2025
AB - The discrepancy in the attosecond time delay between theory and experiment near the 3𝑠 Cooper minimum (CM) of Ar is addressed. It is found that inclusion of the relaxation effects in the time delay difference between Ar 3𝑠 and 3𝑝 photoionization near the 3𝑠 CM dramatically alters the 3𝑠 time delay and brings the theory into substantial agreement with experiment using the relativistic-random-phase approximation with relaxation. The key point is that 3𝑠 photoionization is dominated by interchannel coupling in this region and the interchannel coupling matrix elements were found to be considerably altered by the inclusion of relaxation. This implies that relaxation should be important for any atomic or molecular transition that is dominated by interchannel coupling.
LB - PUB:(DE-HGF)16
DO - DOI:10.1103/PhysRevA.111.052805
UR - https://bib-pubdb1.desy.de/record/646066
ER -