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@ARTICLE{Paulus:645886,
author = {Paulus, Daniel and Linz, Mario and Hansen, Anna-Lena and
van Smaalen, Sander and Moos, Ralf and Ulrich, Anke Silvia
and Schoenauer-Kamin, Daniela},
title = {{S}tructure matters: {A} synchrotron study reveals how
crystallite structure influences the deposition mechanism
for the powder aerosol deposition method},
journal = {Journal of the European Ceramic Society},
volume = {46},
number = {7},
issn = {0955-2219},
address = {Amsterdam [u.a.]},
publisher = {Elsevier Science},
reportid = {PUBDB-2026-00666},
pages = {118127},
year = {2026},
abstract = {Powder aerosol deposition (PAD or ADM) is a coating
technique to produce ceramic films at room temperature.
Although the deposition mechanism has been clarified in some
respects, unanswered questions remain. The present work
reports films of titanium oxide, which forms a typical PAD
microstructure, and films of incommensurate misfit-layered
calcium cobalt oxide (Ca$_3$Co$_4$O$_{9-δ}$, CCO-349),
which forms a atypical film. For this work, films made of
these two materials were examined using X-ray diffraction
with synchrotron radiation and a scanning electron
microscopy. It turned out that due to its aperiodic crystal
structure, CCO-349 can be deformed more easily than
conventional technical ceramics like TiO$_2$. The
deformation occurs when the layers in the crystal slide in
the direction of the misfit. As a result, it is unnecessary
to break the crystals, and a larger crystallite size remains
in the film. Therefore, PAD films of CCO-349 have a
different microstructure.},
cin = {FS DOOR-User},
ddc = {660},
cid = {$I:(DE-H253)FS_DOOR-User-20241023$},
pnm = {6G3 - PETRA III (DESY) (POF4-6G3) / FS-Proposal: I-20230953
(I-20230953) / FS-Proposal: I-20240866 (I-20240866) / DFG
project G:(GEPRIS)544448150 - PAD-Flex-TEG: Direkt aus dem
Pulver kaltabgeschiedene nanokristalline µm-dicke
Bismuttellurid-Schichten für flexible thermoelektrische
Generatoren (544448150) / FestBatt-Oxide - Materialplattform
'Oxide' im Rahmen des Kompetenzclusters für
Festkörperbatterien (13XP0173A)},
pid = {G:(DE-HGF)POF4-6G3 / G:(DE-H253)I-20230953 /
G:(DE-H253)I-20240866 / G:(GEPRIS)544448150 /
G:(BMBF)13XP0173A},
experiment = {EXP:(DE-H253)P-P02.1-20150101},
typ = {PUB:(DE-HGF)16},
doi = {10.1016/j.jeurceramsoc.2026.118127},
url = {https://bib-pubdb1.desy.de/record/645886},
}