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000644465 1001_ $$0P:(DE-H253)PIP1083735$$aDey, Jayjit Kumar$$b0
000644465 245__ $$aAn unconventional pathway to correlate the octahedral tilt coupling and spin-orbit reconstruction at oxide interfaces
000644465 260__ $$a[London]$$bSpringer Nature$$c2026
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000644465 520__ $$aThe direct experimental probing and detailed imaging of octahedral tilt, along with the control of magnetic ground state and spin-orbit occupancies in an artificially engineered heterointerface through the strain manipulation via interface engineering, is the long-standing challenging issue addressed here. We introduce an innovative methodology to measure the projected O-O-O angles (O-O-Oproj) between the neighboring in-plane BO6 octahedra of perovskite oxide (ABO3), demonstrating a precise quantification of strain-manipulated octahedral tilt in atomically engineered LaCoO3 (LCO)/La0.7Sr0.3MnO3 (LSMO) bilayer interfaces. The pronounced octahedral tilt on SrTiO3 (STO) substrate (tensile strain) compared to LaAlO3 (LAO) substrate (compressive strain) correlates to the magnetism especially within the framework of bond angle geometry and spin-charge-orbital reconstructions, contrasting with individual single-phase films. Interfacial orbital reconstruction, Co/Mn antiferromagnetic coupling and their strain manipulation are quantified through X-ray linear dichroism (XLD) and X-ray magnetic circular dichroism (XMCD) measurements, further confirmed by both molecular orbital theory and Goodenough-Kanamori-Anderson rules. First principles calculations unveil a higher (lower) magnetic moment of individual magnetic atoms with tensile (compressive) strain, including unusual interfacial antiferromagnetism arising d-orbital occupations, and bond angle geometry. This endeavor paves a potential method to manipulate the octahedral tilt to tailor emergent phenomena at heterointerfaces via atomically precise strain-interface engineering.
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000644465 7001_ $$aJagadish, Koushik$$b1
000644465 7001_ $$00000-0003-3386-4289$$aBandyopadhyay, Arka$$b2
000644465 7001_ $$0P:(DE-H253)PIP1086088$$aChowdhury, Sourav$$b3
000644465 7001_ $$0P:(DE-H253)PIP1083334$$aHoesch, Moritz$$b4
000644465 7001_ $$00000-0003-4895-8114$$aValvidares, Manuel$$b5
000644465 7001_ $$0P:(DE-H253)PIP1106344$$aAhlawat, Anju$$b6
000644465 7001_ $$0P:(DE-H253)PIP1008946$$aAfaneh, Feras$$b7
000644465 7001_ $$0P:(DE-H253)PIP1107391$$aKeshri, Aryan$$b8
000644465 7001_ $$aRoul, Basanta$$b9
000644465 7001_ $$aKrupanidhi, Saluru Baba$$b10
000644465 7001_ $$0P:(DE-H253)PIP1015097$$aGupta, Mukul$$b11
000644465 7001_ $$aChoudhary, Ram Janay$$b12
000644465 7001_ $$0P:(DE-HGF)0$$aVenkatesan, Thirumalai$$b13$$eCorresponding author
000644465 7001_ $$00000-0003-0127-7047$$aNarayan, Awadhesh$$b14
000644465 7001_ $$00000-0003-0012-046X$$aRavishankar, N.$$b15
000644465 7001_ $$0P:(DE-H253)PIP1027186$$aDas, Sujit$$b16$$eCorresponding author
000644465 773__ $$0PERI:(DE-600)2553671-0$$a10.1038/s41467-025-67042-7$$gVol. 17, no. 1, p. 332$$n1$$p332$$tNature Communications$$v17$$x2041-1723$$y2026
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