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| 001 | 643617 | ||
| 005 | 20260209140538.0 | ||
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| 245 | _ | _ | |a Stability of the collinear up-up-down-down magnetic ordering in Ca$_3$CoMnO$_6$ |
| 260 | _ | _ | |a Woodbury, NY |c 2025 |b Inst. |
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| 520 | _ | _ | |a Ca$_3$CoMnO$_6$ −xMnxO6 is a quasi-one-dimensional Ising chain magnet with a unique collinear up-up-down-down(↑↑↓↓) magnetic ordering, that gives rise to ferroelectricity below the Néel temperature of 13 K. This uniquelong-range magnetic ordering, however, was argued to get stabilized only with Co excess (i.e., x < 1.0) nonstoichiometric Ca$_3$CoMnO$_6$ , and not so for the chemically stoichiometric compound x = 1.0. Combining severalexperiments along with first-principles density-functional-based calculations, we elucidate that this unique↑↑↓↓ magnetic ordering can be stabilized even in the stoichiometric Ca$_3$CoMnO$_6$ (i.e., x = 1.0) compound,albeit through the presence of optimum cationic positional disorder, where some Mn and Co ions occupy thetrigonal-prismatic (Co sites for the ordered case) and octahedral (Mn-sites for the ordered one) sites respectivelythrough relative tuning of the various magnetic exchange interactions. Specifically, the relative energy stabilityof the ↑↑↓↓ magnetic order in Ca3$_3$CoMnO$_6$ exhibits a nonmonotonic dependency on the extent of cationicdisorder with a maximum of around 16% disorder. Thus our study helps to elucidate the mechanism thatleads to stabilization of this unique functional ↑↑↓↓ magnetic ordering in this promising class of multiferroiccompounds. |
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| 700 | 1 | _ | |a Patra, Krishnendu |b 1 |
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| 773 | _ | _ | |a 10.1103/j9r9-9h3q |g Vol. 112, no. 21, p. 214448 |0 PERI:(DE-600)2844160-6 |n 21 |p 214448 |t Physical review / B |v 112 |y 2025 |x 2469-9950 |
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