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@ARTICLE{Pal:643617,
author = {Pal, Pratap and Patra, Krishnendu and Nandy, Subhajit and
Mahana, Sudipta and Dey, Jayjit Kumar and Chatterjee, Souvik
and Prajapat, C. L. and Paramanik, Tapas and Topwal, Dinesh
and Das, Amitabh and Mahadevan, Priya and Choudhury, Debraj},
title = {{S}tability of the collinear up-up-down-down magnetic
ordering in {C}a$_3${C}o{M}n{O}$_6$},
journal = {Physical review / B},
volume = {112},
number = {21},
issn = {2469-9950},
address = {Woodbury, NY},
publisher = {Inst.},
reportid = {PUBDB-2026-00314},
pages = {214448},
year = {2025},
abstract = {Ca$_3$CoMnO$_6$ −xMnxO6 is a quasi-one-dimensional Ising
chain magnet with a unique collinear
up-up-down-down(↑↑↓↓) magnetic ordering, that gives
rise to ferroelectricity below the Néel temperature of 13
K. This uniquelong-range magnetic ordering, however, was
argued to get stabilized only with Co excess (i.e., x < 1.0)
nonstoichiometric Ca$_3$CoMnO$_6$ , and not so for the
chemically stoichiometric compound x = 1.0. Combining
severalexperiments along with first-principles
density-functional-based calculations, we elucidate that
this unique↑↑↓↓ magnetic ordering can be stabilized
even in the stoichiometric Ca$_3$CoMnO$_6$ (i.e., x = 1.0)
compound,albeit through the presence of optimum cationic
positional disorder, where some Mn and Co ions occupy
thetrigonal-prismatic (Co sites for the ordered case) and
octahedral (Mn-sites for the ordered one) sites
respectivelythrough relative tuning of the various magnetic
exchange interactions. Specifically, the relative energy
stabilityof the ↑↑↓↓ magnetic order in
Ca3$_3$CoMnO$_6$ exhibits a nonmonotonic dependency on the
extent of cationicdisorder with a maximum of around 16\%
disorder. Thus our study helps to elucidate the mechanism
thatleads to stabilization of this unique functional
↑↑↓↓ magnetic ordering in this promising class of
multiferroiccompounds.},
cin = {DOOR ; HAS-User / FS-PETRA-S},
ddc = {530},
cid = {I:(DE-H253)HAS-User-20120731 /
I:(DE-H253)FS-PETRA-S-20210408},
pnm = {632 - Materials – Quantum, Complex and Functional
Materials (POF4-632) / 6G3 - PETRA III (DESY) (POF4-6G3) /
INDIA-DESY - INDIA-DESY Collaboration
$(2020_Join2-INDIA-DESY)$},
pid = {G:(DE-HGF)POF4-632 / G:(DE-HGF)POF4-6G3 /
$G:(DE-HGF)2020_Join2-INDIA-DESY$},
experiment = {EXP:(DE-H253)P-P64-20150101},
typ = {PUB:(DE-HGF)16},
doi = {10.1103/j9r9-9h3q},
url = {https://bib-pubdb1.desy.de/record/643617},
}