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000643617 1001_ $$0P:(DE-HGF)0$$aPal, Pratap$$b0
000643617 245__ $$aStability of the collinear up-up-down-down magnetic ordering in Ca$_3$CoMnO$_6$ 
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000643617 520__ $$aCa$_3$CoMnO$_6$ −xMnxO6 is a quasi-one-dimensional Ising chain magnet with a unique collinear up-up-down-down(↑↑↓↓) magnetic ordering, that gives rise to ferroelectricity below the Néel temperature of 13 K. This uniquelong-range magnetic ordering, however, was argued to get stabilized only with Co excess (i.e., x < 1.0) nonstoichiometric Ca$_3$CoMnO$_6$ , and not so for the chemically stoichiometric compound x = 1.0. Combining severalexperiments along with first-principles density-functional-based calculations, we elucidate that this unique↑↑↓↓ magnetic ordering can be stabilized even in the stoichiometric Ca$_3$CoMnO$_6$  (i.e., x = 1.0) compound,albeit through the presence of optimum cationic positional disorder, where some Mn and Co ions occupy thetrigonal-prismatic (Co sites for the ordered case) and octahedral (Mn-sites for the ordered one) sites respectivelythrough relative tuning of the various magnetic exchange interactions. Specifically, the relative energy stabilityof the ↑↑↓↓ magnetic order in Ca3$_3$CoMnO$_6$  exhibits a nonmonotonic dependency on the extent of cationicdisorder with a maximum of around 16% disorder. Thus our study helps to elucidate the mechanism thatleads to stabilization of this unique functional ↑↑↓↓ magnetic ordering in this promising class of multiferroiccompounds. 
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000643617 7001_ $$aPatra, Krishnendu$$b1
000643617 7001_ $$0P:(DE-H253)PIP1108447$$aNandy, Subhajit$$b2$$udesy
000643617 7001_ $$0P:(DE-H253)PIP1028875$$aMahana, Sudipta$$b3
000643617 7001_ $$0P:(DE-H253)PIP1083735$$aDey, Jayjit Kumar$$b4$$udesy
000643617 7001_ $$0P:(DE-H253)PIP1020128$$aChatterjee, Souvik$$b5
000643617 7001_ $$aPrajapat, C. L.$$b6
000643617 7001_ $$00000-0002-8136-8039$$aParamanik, Tapas$$b7
000643617 7001_ $$0P:(DE-H253)PIP1028903$$aTopwal, Dinesh$$b8
000643617 7001_ $$00000-0002-0849-6587$$aDas, Amitabh$$b9
000643617 7001_ $$0P:(DE-HGF)0$$aMahadevan, Priya$$b10
000643617 7001_ $$0P:(DE-H253)PIP1114226$$aChoudhury, Debraj$$b11$$eCorresponding author
000643617 773__ $$0PERI:(DE-600)2844160-6$$a10.1103/j9r9-9h3q$$gVol. 112, no. 21, p. 214448$$n21$$p214448$$tPhysical review / B$$v112$$x2469-9950$$y2025
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