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@ARTICLE{Turak:642766,
author = {Turak, Onur and Gagsteiger, Andreas and Upadhyay, Ashank
and Kriegel, Mark and Salein, Peter and Böhnke-Brandt,
Stefanie and Agarwal, Seema and Borchert, Erik and Höcker,
Birte},
title = {{A} third type of {PET}ase from the marine
{H}alopseudomonas lineage},
journal = {Protein science},
volume = {34},
number = {10},
issn = {0961-8368},
address = {Hoboken, NJ},
publisher = {Wiley},
reportid = {PUBDB-2025-05615},
pages = {e70305},
year = {2025},
abstract = {The enzymatic degradation of polyethylene terephthalate
(PET) offers a sustainable solution for PET recycling. Over
the past two decades, more than 100 PETases have been
characterized, primarily exhibiting similar sequences and
structures. Here, we report PET-degrading α/β hydrolases,
including HaloPETase1 from the marine Halopseudomonas
lineage, thereby extending the narrow sequence space by
novel features at the active site. The crystal structure of
HaloPETase1 was determined to a resolution of 1.16 Å,
revealing a unique active site architecture and a lack of
the canonical π-stacking clamp found in PETases so far.
Further, variations in active site composition and loop
structures were observed. Additionally, we found five more
enzymes from the same lineage, two of which have a high
similarity to type IIa bacterial PETases, while the other
three resemble HaloPETase1. All these enzymes exhibited high
salt tolerance ranging from 2.5 to 5 M NaCl, leading to
higher total product releases upon PET degradation at 40 or
50°C. Based on these findings, we propose an extension of
the existing PETase classification system to include type
III PETases.},
cin = {EMBL-User},
ddc = {610},
cid = {I:(DE-H253)EMBL-User-20120814},
pnm = {6G3 - PETRA III (DESY) (POF4-6G3) / SFB 1357 C03 -
Enzymatischer Abbau synthetischer Polymere (C03)
(419410411)},
pid = {G:(DE-HGF)POF4-6G3 / G:(GEPRIS)419410411},
experiment = {EXP:(DE-H253)P-P13-20150101},
typ = {PUB:(DE-HGF)16},
doi = {10.1002/pro.70305},
url = {https://bib-pubdb1.desy.de/record/642766},
}