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@ARTICLE{Schnorr:641792,
      author       = {Schnorr, Kirsten and Augustin, Sven and Saalmann, Ulf and
                      Schmid, Georg and Rouzée, Arnaud and Obaid, Razib and
                      AlHaddad, Andre and Berrah, Nora and Blaga, Cosmin I. and
                      Bostedt, Christoph and Cardosa-Gutierrez, Manuel and Carini,
                      Gabriella and Coffee, Ryan and DiMauro, Louis F. and Hart,
                      Philip and Ito, Yuta and Kubicek, Katharina and Kumagai,
                      Yoshiaki and Küpper, Jochen and Lai, Yu Hang and
                      Lindenblatt, Hannes and Livingstone, Ruth A. and Meister,
                      Severin and Moshammer, Robert and Motomura, Koji and
                      Möller, Thomas and Nakahara, Kaz and Osipov, Timur and
                      Pandey, Gaurav and Ray, Dipanwita and Remacle, Francoise and
                      Rolles, Daniel and Rost, Jan Michael and Schlichting, Ilme
                      and Schmidt, Rüdiger and Techert, Simone and Trost, Florian
                      and Ueda, Kiyoshi and Ullrich, Joachim and Vrakking, Marc J.
                      J. and Zimmermann, Julian and Schulz, Claus Peter and
                      Pfeifer, Thomas},
      title        = {{V}isualizing the strong field–induced molecular breakup
                      of {C}60 via x-ray diffraction},
      journal      = {Science advances},
      volume       = {11},
      number       = {47},
      issn         = {2375-2548},
      address      = {Washington, DC [u.a.]},
      publisher    = {Assoc.},
      reportid     = {PUBDB-2025-05202},
      pages        = {eadz1900},
      year         = {2025},
      abstract     = {Laser-driven dynamics in polyatomic molecules poses a
                      complex many-body problem. Understanding intense
                      light-matter interaction is crucial for steering
                      intramolecular quantum dynamical processes. Here, we record
                      time-resolved x-ray diffraction images of molecules during
                      and after their interaction with intense near-infrared
                      fields, giving direct access to structural changes of the
                      molecules and their fragmentation in real time. Tuning the
                      intensity of the excitation pulses, we uncover a transition
                      from a weak-field regime of excited but stable molecules to
                      a high-field regime dominated by Coulomb explosion. In the
                      transition region, the molecules expand by up to $50\%$ of
                      their initial size within just 140 fs, with major
                      fragmentation only setting in afterward. This work
                      demonstrates that x-ray diffractive imaging is capable of
                      retrieving time-resolved structural information of large
                      molecules reshaped by intense laser fields. Laser-driven
                      fragmentation is a first step toward observing molecular
                      processes modified by laser fields of increasing intensity.},
      cin          = {FS-SCS / FS-CFEL-CMI / UNI/CUI / UNI/EXP},
      ddc          = {500},
      cid          = {I:(DE-H253)FS-SCS-20131031 /
                      I:(DE-H253)FS-CFEL-CMI-20220405 /
                      $I:(DE-H253)UNI_CUI-20121230$ /
                      $I:(DE-H253)UNI_EXP-20120731$},
      pnm          = {631 - Matter – Dynamics, Mechanisms and Control
                      (POF4-631) / SFB 1073 C02 - In-situ hochauflösende
                      Untersuchung des aktiven Zustands bei der (photo-)
                      elektrochemischen Wasserspaltung (C02) (240172646) / AIM,
                      DFG project G:(GEPRIS)390715994 - EXC 2056: CUI: Advanced
                      Imaging of Matter (390715994) / DFG project
                      G:(GEPRIS)194651731 - EXC 1074: Hamburger Zentrum für
                      ultraschnelle Beobachtung (CUI): Struktur, Dynamik und
                      Kontrolle von Materie auf atomarer Skala (194651731) / DFG
                      project G:(GEPRIS)390900948 - EXC 2181: STRUKTUREN: Emergenz
                      in Natur, Mathematik und komplexen Daten (390900948)},
      pid          = {G:(DE-HGF)POF4-631 / G:(GEPRIS)240172646 /
                      G:(GEPRIS)390715994 / G:(GEPRIS)194651731 /
                      G:(GEPRIS)390900948},
      experiment   = {EXP:(DE-MLZ)External-20140101},
      typ          = {PUB:(DE-HGF)16},
      doi          = {10.1126/sciadv.adz1900},
      url          = {https://bib-pubdb1.desy.de/record/641792},
}