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@ARTICLE{Mollick:641738,
author = {Mollick, Samraj and Morgante, Carmelo and Christensen,
Anders K. R. and Finkler, Jonas A. and Youngman, Randall E.
and Nielsen, Anders B. and Lu, Ronghui and Sørensen, Søren
S. and Johansen, Morten and Karlsen, Martin Aaskov and
Stathopoulos, Vassilis N. and Lock, Nina and Nielsen, Niels
Chr. and Boffa, Vittorio and Smedskjaer, Morten M.},
title = {{S}elective mineral recovery from seawater by
ion-exchangeable metal-organic framework glasses},
reportid = {PUBDB-2025-05149},
year = {2025},
note = {We acknowledge the Deutsche Forschungsgemeinschaft (DFG)
(withinthe SPP 2196: grant numbers GR 5505/3-1, RI
1551/15-2, RI 1551/12-2,RI1551/22-1, OL 462/4-2, OL 462/7-1,
MA 2359/38-1 and HA 4382/16-1)and the Bundesministerium für
Bildung und Forschung (BMBF) (grantnumber 01DP20008) for
financial support.},
abstract = {The transition to clean energy and sustainable technologies
necessitates securing precious metals, yet traditional
land-based mining is increasingly unsustainable. Seawater
holds immense potential as a mineral source, but its
intricate ionic composition limits current extraction
techniques. Here, we report a family of ion-exchangeable
materials by grafting phosphate groups onto metal-organic
framework glasses, followed by precise heat and aqueous
treatments. This process introduces facile exchangeable ions
and exposes active functional groups. Based on these
structural features, the materials exhibit superior
performance in selective recovery of magnesium and lithium
from various natural seawater samples, surpassing a typical
commercial resin in uptake rate, capacity, and
recyclability. Our work presents a promising route for
designing efficient adsorbents to extract valuable minerals
from unconventional sources and help to secure the raw
materials vital for a low-carbon future.},
cin = {DOOR ; HAS-User / FS-PETRA-D},
cid = {I:(DE-H253)HAS-User-20120731 /
I:(DE-H253)FS-PETRA-D-20210408},
pnm = {632 - Materials – Quantum, Complex and Functional
Materials (POF4-632) / 6G3 - PETRA III (DESY) (POF4-6G3) /
05K19VTA - Entwicklung einer kompakten Probenumgebung mit
Spin-Coater für in-situ Röntgenstreuung an PETRA III.
(BMBF-05K19VTA) / FOXES - Fully Oxide-based Zero-Emission
and Portable Energy Supply (951774) / TRIUMPH - Triple
junction solar modules based on perovskites and silicon for
high performance, low-cost and small environmental footprint
(101075725) / FS-Proposal: I-20211642 (I-20211642) /
FS-Proposal: II-20190761 (II-20190761) / FS-Proposal:
I-20221269 (I-20221269)},
pid = {G:(DE-HGF)POF4-632 / G:(DE-HGF)POF4-6G3 /
G:(DE-Ds200)BMBF-05K19VTA / G:(EU-Grant)951774 /
G:(EU-Grant)101075725 / G:(DE-H253)I-20211642 /
G:(DE-H253)II-20190761 / G:(DE-H253)I-20221269},
experiment = {EXP:(DE-H253)P-P08-20150101},
typ = {PUB:(DE-HGF)25},
doi = {10.26434/chemrxiv-2025-90l2h-v2},
url = {https://bib-pubdb1.desy.de/record/641738},
}